Influence of Electronic Effect on Methane Catalytic Combustion over PdNi/Al2O3

doi:10.1007/s40242-013-3135-2

Abstract

Abstract:

A series of PdNi/Al₂O₃ catalysts with different compositions was prepared by co-reduction method. The influence of Ni amount on the catalytic combustion of methane was studied. X-ray diffractometry and X-ray photo-electron spectroscopy were employed to characterize the dispersion and electronic state of the active phase. Tempe-rature-programmed oxidation was carried out to study the thermal stability affected by Ni doping. It has been demonstrated that Ni addition changed particle size and oxidation state of PdO_x. The results indicate that the promotion of Ni to the Pd/Al₂O₃ resulted from both size effect and electronic effect. In addition, the thermal stability of the Ni-doped catalysts were enhanced.

Key words: Methane combustion, Palladium, Nickel, Size effect, Electronic effect

PAN Xi-qiang, ZHANG Yi-bo, ZHANG Bin, MIAO Zhen-zhen, WU Tian-xiao, YANG Xiang-guang. Influence of Electronic Effect on Methane Catalytic Combustion over PdNi/Al₂O₃[J]. Chemical Research in Chinese Universities, 2013, 29(5): 952-955.

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Influence of Electronic Effect on Methane Catalytic Combustion over PdNi/Al₂O₃

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