Progress on High Voltage PEO-based Polymer Solid Electrolytes in Lithium Batteries

doi:10.1007/s40242-022-2065-2

Abstract

Abstract: Polymer electrolytes have attracted great interest for next-generation lithium-based batteries on account of safety and high energy density. In this review, we assess recent progress on the design of poly(ethylene oxide)(PEO)-based solid polymer electrolytes in high voltage lithium batteries and identify possible side reactions between PEO-based electrolytes and existing cathodes. We provide an overview of the ways to enhance high voltage resistance of PEO-based electrolytes. Those include components blend, molecular design and interface modification. With these efforts, we want to present new insights into rational design of PEO-based electrolytes to develop solid-state lithium batteries for advanced performance.

Key words: Poly(ethylene oxide), Lithium battery, High voltage, Molecular design, Interface modification

HOU Wenhui, OU Yu and LIU Kai. Progress on High Voltage PEO-based Polymer Solid Electrolytes in Lithium Batteries[J]. Chemical Research in Chinese Universities, 2022, 38(3): 735-743.

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