Stabilizing High-voltage Cathode Materials for Next-generation Li-ion Batteries

doi:10.1007/s40242-020-9103-8

Abstract

Abstract: The pressing demand for high-energy/power lithium-ion batteries requires the deployment of cathode materials with higher capacity and output voltage. Despite more than ten years of research, high-voltage cathode mate-rials, such as high-voltage layered oxides, spinel LiNi_0.5Mn_1.5O₄, and high-voltage polyanionic compounds still cannot be commercially viable due to the instabilities of standard electrolytes, cathode materials, and cathode electrolyte interphases under high-voltage operation. This paper summarizes the recent advances in addressing the surface and interface issues haunting the application of high-voltage cathode materials. The understanding of the limitations and advantages of different modification protocols will direct the future endeavours on advancing high-energy/power lithium-ion batteries.

Key words: High voltage, Cathode material, Surface engineering, Cathode electrolyte interphase, Cycling stability, Lithium ion battery

ZHU Xiaobo, Tobias Schulli, WANG Lianzhou. Stabilizing High-voltage Cathode Materials for Next-generation Li-ion Batteries[J]. Chemical Research in Chinese Universities, 2020, 36(1): 24-32.

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