Rapid Degrading Carbamazepine in a Novel Advanced Oxidation Process of Bisulfite Activated by Lithium Cobaltate Recovered from Spent Lithium-ion Battery

doi:10.1007/s40242-024-3237-z

Chemical Research in Chinese Universities ›› 2024, Vol. 40 ›› Issue (1): 127-135.doi: 10.1007/s40242-024-3237-z

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Rapid Degrading Carbamazepine in a Novel Advanced Oxidation Process of Bisulfite Activated by Lithium Cobaltate Recovered from Spent Lithium-ion Battery

YAN Jiali^1,2,3, YANG Kaiying^1,2,3, WANG Xi^1,2,3, ZHAI Jinli^1,2,3, ZHU Wenjie^1,2,3, YANG Daoli¹, LUO Yongming^1,2,3, GAO Xiaoya^1,2,3

1. Faculty of Environmental Science and Engineering, Kunming University of Science and Technology, Kunming 650500, P. R. China;
2. Innovation Team for Volatile Organic Compounds Pollutants Control and Resource Utilization of Yunnan Province, Kunming 650500, P. R. China;
3. Higher Educational Key Laboratory for Odorous Volatile Organic Compounds Pollutants Control of Yunnan Province, Kunming 650500, P. R. China

Received:2023-10-26 Online:2024-02-01 Published:2024-01-24
Contact: GAO Xiaoya E-mail:gaoxiaoyaya@kust.edu.cn
Supported by:
This work was supported by the National Natural Science Foundation of China (Nos. 42067057, 42367060), the Science and Technology Plan Project of Yunnan Provincial Science and Technology Department, China (No. 202101AT070087), and the High-level Scientific Research Foundation for Talent Introduction of Kunming University of Science and Technology, China (No. 10978172).

Abstract

Abstract: Maximizing the sustainable recycling of spent lithium-ion batteries (LIBs) shows economic and environmental significance. This study recovered lithium cobaltate (LiCoO₂, LCO) from spent LIBs cathode powder. The recovered LCO was then combined with NaHSO₃ to remove refractory organic pollutants of carbamazepine (CBZ) in water. The degradation of CBZ reached 80.0% within 60 min, by ¹O₂, SO₄^-·, ^·OH and O₂^-· generated in the LCO/NaHSO₃ reaction. The electron transfer between Co (III) and Co (II) was beneficial to the generation of free radicals. The LCO/NaHSO₃ degraded CBZ effectively in both secondary outlet water and tap water. However, high concentrations of inorganic ions (Cl^‒, HCO₃^-, HPO₄^2-, SO₄^2-, NO₃^-) and natural organic matter (humic acid, HA) could inhibit the degradation of CBZ. After three cycles, the stability of the LCO/NaHSO₃ system was demonstrated by the maintained high efficiency in the degradation of CBZ. The obtained data indicate that the LCO/NaHSO₃ system holds great application potential in the field of advanced oxidation degradation of pollutants.

Key words: Spent lithium-ion battery, Lithium cobaltate, Carbamazepine, NaHSO₃, Advanced oxidation

YAN Jiali, YANG Kaiying, WANG Xi, ZHAI Jinli, ZHU Wenjie, YANG Daoli, LUO Yongming, GAO Xiaoya. Rapid Degrading Carbamazepine in a Novel Advanced Oxidation Process of Bisulfite Activated by Lithium Cobaltate Recovered from Spent Lithium-ion Battery[J]. Chemical Research in Chinese Universities, 2024, 40(1): 127-135.

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Rapid Degrading Carbamazepine in a Novel Advanced Oxidation Process of Bisulfite Activated by Lithium Cobaltate Recovered from Spent Lithium-ion Battery

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