3D Tungsten Trioxide Nanosheets as Optoelectronic Materials for On-chip Quantification of Global Antioxidant Capacity

doi:10.1007/s40242-020-0234-8

Chemical Research in Chinese Universities ›› 2021, Vol. 37 ›› Issue (3): 763-771.doi: 10.1007/s40242-020-0234-8

• Articles • Previous Articles Next Articles

3D Tungsten Trioxide Nanosheets as Optoelectronic Materials for On-chip Quantification of Global Antioxidant Capacity

DAI Mengjiao^1,2, MA Weiguang³, HAN Fangjie^1,2, HAN Dongfang⁴, HAN Lipeng⁴, WANG Wei^1,4, ZHAO Bolin⁴, HAN Dongxue^1,2,4, NIU Li^1,2,4, WANG Zhenxin^1,2

1. State Key Laboratory of Electroanalytical Chemistry, c/o Engineering Laboratory for Modern Analytical Techniques, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P. R. China;
2. University of Science and Technology of China, Hefei 230026, P. R. China;
3. Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, P. R. China;
4. Center for Advanced Analytical Science, c/o School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou 510006, P. R. China

Received:2020-07-14 Revised:2020-09-03 Online:2021-06-01 Published:2021-05-31
Contact: MA Weiguang, WANG Wei E-mail:wgma@dicp.ac.cn;wangw@gzhu.edu.cn
Supported by:
This work was supported by the National Natural Science Foundation of China(Nos.21527806, 21627809, 21727815), the Project of the Department of Science and Techniques of Guangdong Province, China(No.2019B010933001) and the Project of the Department of Science and Techniques of Jilin Province, China(Nos.20170442014SC, 20170203004SF, 20170101183JC, 20180201021GX).

Abstract

Abstract: The photoelectrochemical properties of semiconductors mainly depend on the size and shape of the corresponding nanoparticles. Herein, 3D WO₃ nanosheets were controllably synthesized with the aid of polyethyleneimine, which presents enhanced photocurrent responses. Based on this excellent photoelectrochemical property, a photoelectrochemical chip was prepared by lithography technology for the smart monitoring of the antioxidant capacity(AC) in red wine and exhibits a series of advantages inclu-ding rapid response time, high sensitivity, and long-lasting stability. The mechanism of the present photoelectrochemical sensing was explored and shows a single electron transfer reaction. Furthermore, only 200 μL of samples are required for one testing, which demonstrates that the present photoelectrochemical chip can be potentially integrated with a portable commercial device(such as a mobile phone) for further research and development of food and drug supervision.

Key words: 3D tungsten trioxide nanosheet, Photoelectrochemical chip, Antioxidant capacity assessment, Red wine assessment, Gallic acid

DAI Mengjiao, MA Weiguang, HAN Fangjie, HAN Dongfang, HAN Lipeng, WANG Wei, ZHAO Bolin, HAN Dongxue, NIU Li, WANG Zhenxin. 3D Tungsten Trioxide Nanosheets as Optoelectronic Materials for On-chip Quantification of Global Antioxidant Capacity[J]. Chemical Research in Chinese Universities, 2021, 37(3): 763-771.

References 48

[1]	Tang J., Xiong P. Y., Li J. J., Cheng Y., Tian X. C., Chen Y., Sun Y. F., Tang D. P., Sens. Actuator B:Chem., 2019, 297, 8
[2]	Huang D., Wang L., Zhan Y., Zou L. N., Ye B. X., Biosens. Bioelectron., 2019, 140, 183
[3]	Xu R., Wei D., Du B., Cao W., Fan D. W., Zhang Y., Wei Q., Ju H. X., Biosens. Bioelectron., 2018, 122, 37
[4]	Li H. Y., Wang J., Wang X., Lin H. Y., Li F., ACS Appl. Mater. Interfaces, 2019, 11, 16958
[5]	Wang C., Wu T., Wang X., Wei Q. X., Wang Y. Y., Li C. Y., Sun D., Sens. Actuator B:Chem., 2019, 297, 7
[6]	Long Y. T., Kong C., Li D. W., Li Y., Chowdhury S., Tian H., Small, 2011, 7, 1624
[7]	Ma W. G., Wang L. N., Zhang N., Han D. X., Dong X., Niu L., Anal. Chem., 2015, 87, 4844
[8]	Wang L. N., Han D. X., Ni S., Ma W. G., Wang W., Niu L., Chem. Sci., 2015, 6, 6632
[9]	Zhang X. Y., Liu S. G., Zhang W. J., Wang X. H., Han L., Ling Y., Li N. B., Luo H. Q., Sens. Actuator B:Chem., 2019, 297, 9
[10]	Zhao W.-W., Xu J.-J., Chen H.-Y., Chem. Soc. Rev., 2015, 44, 729
[11]	Mahadik M. A., An G. W., David S., Choi S. H., Cho M., Jang J. S., Appl. Surf. Sci., 2017, 426, 833
[12]	Qiu L. Y., Wang Q. Y., Liu Z. Y., Zhao Q. Q., Tian X. Y., Li H. L., Gao S. M., Sep. Purif. Technol., 2018, 207, 206
[13]	Jiang Z. Y., Liang X. Z., Zheng H. L., Liu Y. Y., Wang Z. Y., Wang P., Zhang X. Y., Qin X. Y., Dai Y., Whangbo M. H., Huang B. B., Appl. Cata. B, 2017, 219, 209
[14]	Harman T. C., Taylor P. J., Walsh M. P., LaForge B. E., Science, 2002, 297, 2229
[15]	Wang S. T., Feng X. J., Yao J. N., Jiang L., Angew. Chem. Int. Ed., 2006, 45, 1264
[16]	Yan J. Q., Wang T., Wu G. J., Dai W. L., Guan N. J., Li L. D., Gong J. L., Adv. Mater., 2015, 27, 1580
[17]	Liu X., Jin A. L., Jia Y. S., Xia T. L., Deng C. X., Zhu M. H., Chen C. F., Chen X. S., Appl. Surf. Sci., 2017, 405, 359
[18]	Wen L., Chen L., Zheng S. M., Zeng J. F., Duan G. X., Wang Y., Wang G. L., Chai Z. F., Li Z., Gao M. Y., Adv. Mater., 2016, 28, 5072
[19]	Cong S., Geng F. X., Zhao Z. G., Adv. Mater., 2016, 28, 10518
[20]	Liu Y., Wygant B. R., Kawashima K., Mabayoje O., Hong T. E., Lee S. G., Lin J., Kim J.-H., Yubuta K., Li W. Z., Li J., Mullins C. B., Appl. Cata. B, 2019, 245, 227
[21]	Wang Z. H., Fan X. X., Li C. J., Men G. L., Han D. M., Gu F. B., ACS Appl. Mater. Interfaces, 2018, 10, 3776
[22]	Liu J.-W., Zheng J., Wang J.-L., Xu J., Li H.-H., Yu S.-H., Nano Lett., 2013, 13, 3589
[23]	Chandra D., Saito K., Yui T., Yagi M., Angew. Chem. Int. Ed., 2013, 52, 12606
[24]	Perera R. M., Bardeesy N., Nature, 2011, 475, 43
[25]	Eberhardt M. V., Lee C. Y., Liu R. H., Nature, 2000, 405, 903
[26]	Han F. J., Song Z. Q., Nawaz M. H., Dai M. J., Han D. F., Han L. P., Fan Y. Y., Xu J. N., Han D. X., Niu L., Anal. Chem., 2019, 91, 10657
[27]	Wang L. N., Liu Z. B., Wang D. D., Ni S., Han D. X., Wang W., Niu L., Biosens. Bioelectron., 2017, 94, 107
[28]	Han D. X., Ma W. G., Wang L. N., Ni S., Zhang N., Wang W., Dong X. D., Niu L., Biosens. Bioelectron., 2016, 75, 458
[29]	Ma W. G., Wang L. N., Zhang N., Han D. X., Dong X., Niu L., Anal. Chem., 2015, 87, 4844
[30]	Wang L. N., Han D. X., Ni S., Ma W. G., Wang W., Niu L., Chem. Sci., 2015, 6, 6632
[31]	Wang K., Li M., Liu Y. N., Gu Y. Z., Li Q. W., Zhang Z. G., Appl. Surf. Sci., 2014, 292, 469
[32]	Ainsworth E. A., Gillespie K. M., Nat. Protoc., 2007, 2, 875
[33]	Brand-Williams W., Cuvelier M. E., Berset C., LWT, 1995, 28, 25
[34]	Ma W. G., Han D. X., Zhang N., Li F. H., Wu T. S., Dong X. D., Niu L., Analyst, 2013, 138, 2335
[35]	Li W. J., Da P. M., Zhang Y. Y., Wang Y. C., Lin X., Gong X. G., Zheng G. F., ACS nano, 2014, 8, 11770
[36]	Santato C., Odziemkowski M., Ulmann M., Augustynski J., J. Am. Chem. Soc., 2001, 123, 10639
[37]	Wang R., Zhang W. T., Zhu W. X., Yan L. Z., Li S. H., Chen K., Hu N., Suo Y., Wang J. L., Chem. Eng. J., 2018, 348, 292
[38]	Kim J. K., Shin K., Cho S. M., Lee T. W., Park J. H., Energy Environ. Sci., 2011, 4, 1465
[39]	Ma W. G., Han D. X., Zhou M., Sun H., Wang L. N., Dong X. D., Niu L., Chemi. Sci., 2014, 5, 3946
[40]	Wang L. N., Ma W. G., Gan S. Y., Han D. Y., Zhang Q. X., Niu L., Anal. Chem., 2014, 86, 10171
[41]	Liu P., Hu D. C. M., Tran T. Q., Jewell D., Duong H. M., Colloid Surface A, 2016, 509, 384
[42]	Kar P., Choudhury A., Sens. Actuators B Chem., 2013, 183, 25
[43]	Benzie I. F. F. B., Choi S. W., Adv. Food Nutr. Res., 2014, 71, 1
[44]	Wright J. S., Johnson E. R., DiLabio G. A., J. Am. Chem. Soc., 2001, 123, 1173
[45]	Leopoldini M., Pitarch I. P., Russo N., Toscano M., J. Phys. Chem. A, 2004, 108, 92
[46]	Zhang N., Ma W. G., Han D. X., Wang L. N., Wu T. S., Talanta, 2015, 144, 551
[47]	Cai Z. X., Rong M. C., Zhao T. T., Zhao L., Wang Y. R., Chen X., J. Electroanal. Chem., 2015, 759, 32
[48]	Kovachev N., Canals A., Escarpa A., Anal. Chem., 2010, 82, 2925

3D Tungsten Trioxide Nanosheets as Optoelectronic Materials for On-chip Quantification of Global Antioxidant Capacity

Knowledge

Abstract

Cite this article

share this article

References 48

Related Articles 2

Recommended Articles

Metrics

Comments

[1]	SONG Yudong, HUANG Hui, HE Dayong, YANG Mei, WANG Hao, ZHANG Hao, LI Jiali, LI Yongxin, WANG Ce. Gallic Acid/2-Hydroxypropyl-β-cyclodextrin Inclusion Complexes Electrospun Nanofibrous Webs: Fast Dissolution, Improved Aqueous Solubility and Antioxidant Property of Gallic Acid [J]. Chemical Research in Chinese Universities, 2021, 37(3): 450-455.
[2]	LIU Zuo-jia, LI Dan, NIU Feng-lan. Characterization of Gallic Acid Interaction with Human Serum Albumin by Spectral and Molecular Modeling Methods [J]. Chemical Research in Chinese Universities, 2012, 28(2): 287-290 .