Effect of Preparation Method on the Structural Characteristics of NiO-ZrO2 Oxygen Carriers for Chemical-looping Combustion

doi:10.1007/s40242-019-9189-z

Chemical Research in Chinese Universities ›› 2019, Vol. 35 ›› Issue (6): 1024-1031.doi: 10.1007/s40242-019-9189-z

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Effect of Preparation Method on the Structural Characteristics of NiO-ZrO₂ Oxygen Carriers for Chemical-looping Combustion

LIU Yike^1,2,3, LONG Yanhui³, TANG Yaqin^1,2,3, GU Zhenhua^2,3,4, LI Kongzhai^2,3,4

1. School of Material and Metallurgical Engineering, Guizhou Institute of Technology, Guiyang 550003, P. R. China;
2. Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, P. R. China;
3. State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 650093, P. R. China;
4. Engineering Research Center of Metallurgical Energy Conservation and Emission Reduction, Ministry of Education, Kunming University of Science and Technology, Kunming 650093, P. R. China

Received:2019-07-10 Revised:2019-09-16 Online:2019-12-01 Published:2019-11-29
Contact: GU Zhenhua E-mail:gzhua17@163.com
Supported by:
Supported by the National Natural Science Foundation of China(No.51604137) and the Natural Science Foundation of Guizhou Province, China(No.QianKeHe[2017]1064).

Abstract

Abstract: Chemical-looping combustion(CLC) offers an effective approach for power generation and CO₂ capture. In this work, an NiO-ZrO₂ oxygen carrier prepared by three methods was subjected to an optimal reaction temperature test, an optimal flow test and a cyclic redox reaction test to explore the most suitable reaction conditions. Through comparative analysis, it is noted that the coprecipitation method is not suitable for the preparation of this NiO-ZrO₂ oxygen carrier, while the oxygen carrier prepared by the mechanical mixing method and solution combustion method obtained a higher CH₄ conversion rate and CO₂ selectivity. In addition, these two oxygen carriers also showed high stability during successive CLC testing. Therefore, both the mechanical mixing method and the solution combustion method can be used to prepare NiO-ZrO₂ oxygen carriers.

Key words: Chemical-looping combustion, NiO-ZrO₂ oxygen carrier, Solution combustion method, Mechanical mixing method, Coprecipitation method

LIU Yike, LONG Yanhui, TANG Yaqin, GU Zhenhua, LI Kongzhai. Effect of Preparation Method on the Structural Characteristics of NiO-ZrO₂ Oxygen Carriers for Chemical-looping Combustion[J]. Chemical Research in Chinese Universities, 2019, 35(6): 1024-1031.

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Effect of Preparation Method on the Structural Characteristics of NiO-ZrO₂ Oxygen Carriers for Chemical-looping Combustion

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