Recent Advances of Porous Solids for Ultradilute CO2 Capture

doi:10.1007/s40242-021-1394-x

高等学校化学研究 ›› 2022, Vol. 38 ›› Issue (1): 18-30.doi: 10.1007/s40242-021-1394-x

Recent Advances of Porous Solids for Ultradilute CO₂ Capture

LIU Ru-Shuai, XU Shuang, HAO Guang-Ping, LU An-Hui

State Key Laboratory of Fine Chemicals, Liaoning Key Laboratory for Catalytic Conversion Carbon Resources, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, P. R. China

收稿日期:2021-09-28 修回日期:2021-10-25 出版日期:2022-02-01 发布日期:2021-10-25
通讯作者: HAO Guang-Ping, LU An-Hui E-mail:guangpinghao@dlut.edu.cn;anhuilu@dlut.edu.cn
基金资助:
This work was supported by the National Natural Science Foundation of China (No.21975037), the Cheung Kong Scholars Program of China(No.T2015036), the Fundamental Research Funds for the Central Universities, China[No.DUT18RC(3)075] and the Liao Ning Revitalization Talents Program, China (No.XLYC1807205).

Recent Advances of Porous Solids for Ultradilute CO₂ Capture

LIU Ru-Shuai, XU Shuang, HAO Guang-Ping, LU An-Hui

State Key Laboratory of Fine Chemicals, Liaoning Key Laboratory for Catalytic Conversion Carbon Resources, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, P. R. China

Received:2021-09-28 Revised:2021-10-25 Online:2022-02-01 Published:2021-10-25
Contact: HAO Guang-Ping, LU An-Hui E-mail:guangpinghao@dlut.edu.cn;anhuilu@dlut.edu.cn
Supported by:
This work was supported by the National Natural Science Foundation of China (No.21975037), the Cheung Kong Scholars Program of China(No.T2015036), the Fundamental Research Funds for the Central Universities, China[No.DUT18RC(3)075] and the Liao Ning Revitalization Talents Program, China (No.XLYC1807205).

摘要/Abstract

摘要： The urgency of dealing with global climate change caused by greenhouse gas(GHG) emissions is increasing as the carbon dioxide(CO₂) concentration in the atmosphere has reached a record high value of 416 ppm(parts per million). Technologies that remove CO₂ from the surrounding air(direct air capture, DAC) could result in negative carbon emissions, and thus attracts increasing attention. The steady technical progress in adsorption-based CO₂ separation greatly advanced the DAC, which largely relies on advanced sorbent materials. This review focuses on the latest development of porous solids for air capture; first discussed the main types of sorbents for air capture, which include porous carbons, zeolites, silica materials, and metal-organic frameworks(MOFs), particularly their modified counterparts. Then, we evaluated their performances, including uptake and selectivity under dry and humid CO₂ streams for practical DAC application. Finally, a brief outlook on remaining challenges and potential directions for future DAC development is given.

关键词: Direct air capture, Porous carbon, CO₂ capture, Porous solid, Adsorption

Abstract: The urgency of dealing with global climate change caused by greenhouse gas(GHG) emissions is increasing as the carbon dioxide(CO₂) concentration in the atmosphere has reached a record high value of 416 ppm(parts per million). Technologies that remove CO₂ from the surrounding air(direct air capture, DAC) could result in negative carbon emissions, and thus attracts increasing attention. The steady technical progress in adsorption-based CO₂ separation greatly advanced the DAC, which largely relies on advanced sorbent materials. This review focuses on the latest development of porous solids for air capture; first discussed the main types of sorbents for air capture, which include porous carbons, zeolites, silica materials, and metal-organic frameworks(MOFs), particularly their modified counterparts. Then, we evaluated their performances, including uptake and selectivity under dry and humid CO₂ streams for practical DAC application. Finally, a brief outlook on remaining challenges and potential directions for future DAC development is given.

Key words: Direct air capture, Porous carbon, CO₂ capture, Porous solid, Adsorption

LIU Ru-Shuai, XU Shuang, HAO Guang-Ping, LU An-Hui. Recent Advances of Porous Solids for Ultradilute CO₂ Capture[J]. 高等学校化学研究, 2022, 38(1): 18-30.

LIU Ru-Shuai, XU Shuang, HAO Guang-Ping, LU An-Hui. Recent Advances of Porous Solids for Ultradilute CO₂ Capture[J]. Chemical Research in Chinese Universities, 2022, 38(1): 18-30.

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Recent Advances of Porous Solids for Ultradilute CO₂ Capture

Recent Advances of Porous Solids for Ultradilute CO₂ Capture

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