Covalent Organic Frameworks(COFs) for Sequestration of99TcO4–

doi:10.1007/s40242-022-1447-9

高等学校化学研究 ›› 2022, Vol. 38 ›› Issue (2): 290-295.doi: 10.1007/s40242-022-1447-9

Covalent Organic Frameworks(COFs) for Sequestration of⁹⁹TcO₄^–

DI Zhengyi, MAO Yining, YUAN Heng, ZHOU Yan, JIN Jun, LI Cheng-Peng

College of Chemistry, Tianjin Key Laboratory of Structure and Performance for Functional Molecules, Tianjin Normal University, Tianjin 300387, P. R. China

收稿日期:2021-11-06 修回日期:2021-12-03 出版日期:2022-04-01 发布日期:2022-05-18
通讯作者: LI Cheng-Peng E-mail:hxxylcp@tjnu.edu.cn
基金资助:
This work was supported by the National Natural Science Foundation of China (Nos.22171210, 21771139) and the Program for Innovative Research Team in University of Tianjin, China(No.TD13-5074).

Covalent Organic Frameworks(COFs) for Sequestration of⁹⁹TcO₄^–

DI Zhengyi, MAO Yining, YUAN Heng, ZHOU Yan, JIN Jun, LI Cheng-Peng

College of Chemistry, Tianjin Key Laboratory of Structure and Performance for Functional Molecules, Tianjin Normal University, Tianjin 300387, P. R. China

Received:2021-11-06 Revised:2021-12-03 Online:2022-04-01 Published:2022-05-18
Contact: LI Cheng-Peng E-mail:hxxylcp@tjnu.edu.cn
Supported by:
This work was supported by the National Natural Science Foundation of China (Nos.22171210, 21771139) and the Program for Innovative Research Team in University of Tianjin, China(No.TD13-5074).

摘要/Abstract

摘要： Covalent organic frameworks(COFs), as a class of crystalline porous materials with periodic lattices and porous structures, have received extensive attention in the fields of gas storage and separation, energy storage, catalysis and optoelectronics and so on. However, COFs are still in their infancy in the field of nuclear waste treatment, especially for sequestration of long-live problematic radionuclides, such as ⁹⁹Tc. Battle of decontamination of pertechnetate(TcO₄^–), a main existence of ⁹⁹Tc under aerobic environments, is far from finished. In this review, recent progresses of COFs and some relative materials in the sequestration of pertechnetate, and perspective on surmounting the unmet issues are elucidated.

关键词: Covalent organic framework(COF), Radionuclide sequestration, ⁹⁹TcO₄^–, Adsorption, Anion exchange

Abstract: Covalent organic frameworks(COFs), as a class of crystalline porous materials with periodic lattices and porous structures, have received extensive attention in the fields of gas storage and separation, energy storage, catalysis and optoelectronics and so on. However, COFs are still in their infancy in the field of nuclear waste treatment, especially for sequestration of long-live problematic radionuclides, such as ⁹⁹Tc. Battle of decontamination of pertechnetate(TcO₄^–), a main existence of ⁹⁹Tc under aerobic environments, is far from finished. In this review, recent progresses of COFs and some relative materials in the sequestration of pertechnetate, and perspective on surmounting the unmet issues are elucidated.

Key words: Covalent organic framework(COF), Radionuclide sequestration, ⁹⁹TcO₄^–, Adsorption, Anion exchange

DI Zhengyi, MAO Yining, YUAN Heng, ZHOU Yan, JIN Jun, LI Cheng-Peng. Covalent Organic Frameworks(COFs) for Sequestration of⁹⁹TcO₄^–[J]. 高等学校化学研究, 2022, 38(2): 290-295.

DI Zhengyi, MAO Yining, YUAN Heng, ZHOU Yan, JIN Jun, LI Cheng-Peng. Covalent Organic Frameworks(COFs) for Sequestration of⁹⁹TcO₄^–[J]. Chemical Research in Chinese Universities, 2022, 38(2): 290-295.

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Covalent Organic Frameworks(COFs) for Sequestration of⁹⁹TcO₄^–

Covalent Organic Frameworks(COFs) for Sequestration of⁹⁹TcO₄^–

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