Recent Advances in Biomass-derived Porous Carbon Materials: Synthesis, Composition and Applications

doi:10.1007/s40242-024-3259-6

高等学校化学研究 ›› 2024, Vol. 40 ›› Issue (1): 3-19.doi: 10.1007/s40242-024-3259-6

Recent Advances in Biomass-derived Porous Carbon Materials: Synthesis, Composition and Applications

ZHAI Ziqi¹, LU Yumiao^1,2, LIU Guangyong¹, DING Wei-Lu^1,2, CAO Bobo^1,2, HE Hongyan^1,2,3

1. CAS Key Laboratory of Green Process and Engineering, State Key Laboratory of Mesoscience and Engineering, Beijing Key Laboratory of Ionic Liquids Clean Process, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, P. R. China;
2. University of Chinese Academy of Sciences, Beijing 100049, P. R. China;
3. Longzihu New Energy Laboratory, Zhengzhou Institute of Emerging Industrial Technology, Zhengzhou 450000, P. R. China

收稿日期:2023-11-24 出版日期:2024-02-01 发布日期:2024-01-24
通讯作者: LIU Guangyong, HE Hongyan E-mail:ymlv@ipe.ac.cn;hyhe@ipe.ac.cn
基金资助:
This work was supported by the National Key Research and Development Program of China (No. 2021YFB3802600), the National Natural Science Foundation of China (Nos. 22278396, 22378392, 22178344), the Project of the Youth Innovation Promotion Association, CAS (No. Y2021022), and the Open Research Fund of State Key Laboratory of Mesoscience and Engineering, China (No. MESO-23-D17).

Recent Advances in Biomass-derived Porous Carbon Materials: Synthesis, Composition and Applications

ZHAI Ziqi¹, LU Yumiao^1,2, LIU Guangyong¹, DING Wei-Lu^1,2, CAO Bobo^1,2, HE Hongyan^1,2,3

1. CAS Key Laboratory of Green Process and Engineering, State Key Laboratory of Mesoscience and Engineering, Beijing Key Laboratory of Ionic Liquids Clean Process, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, P. R. China;
2. University of Chinese Academy of Sciences, Beijing 100049, P. R. China;
3. Longzihu New Energy Laboratory, Zhengzhou Institute of Emerging Industrial Technology, Zhengzhou 450000, P. R. China

Received:2023-11-24 Online:2024-02-01 Published:2024-01-24
Contact: LIU Guangyong, HE Hongyan E-mail:ymlv@ipe.ac.cn;hyhe@ipe.ac.cn
Supported by:
This work was supported by the National Key Research and Development Program of China (No. 2021YFB3802600), the National Natural Science Foundation of China (Nos. 22278396, 22378392, 22178344), the Project of the Youth Innovation Promotion Association, CAS (No. Y2021022), and the Open Research Fund of State Key Laboratory of Mesoscience and Engineering, China (No. MESO-23-D17).

摘要/Abstract

摘要： Porous carbon materials (PCMs) play a pivotal role in diverse applications, such as energy storage, adsorption, catalysis, environmental remediation, and microwave adsorption. The selection of carbon precursors, in particular, is crucial for tailoring porous structures with specific functionalities. Biomass, with its rich carbon feedstock, abundant availability, renewability, and versatile structures, has emerged as a promising precursor for porous carbon material synthesis. This review comprehensively summarizes the recent advances in biomass-derived porous carbon materials (BPCMs) encompassing synthetic strategy, morphology, structural composition, and multiple applications. We first review synthetic approaches aiming at regulating porosity, followed by morphological and composition features of BPCMs, with a special emphasis on elucidating the dimensional clarification and heteroatom doping effects. The discussion then extends to the wide-ranging applications of BPCMs, covering energy-related applications and CO₂ adsorption to environmental remediation. Finally, the review outlines the existing challenges and prospects in the field. In summary, this review systematically describes BPCMs and provides valuable guidance for researchers to select and synthesize BPCMs that meet specific functional requirements.

关键词: Biomass, Porous carbon, Pyrolysis, Heteroatom-doping, Supercapacitor, CO₂ adsorption

Abstract: Porous carbon materials (PCMs) play a pivotal role in diverse applications, such as energy storage, adsorption, catalysis, environmental remediation, and microwave adsorption. The selection of carbon precursors, in particular, is crucial for tailoring porous structures with specific functionalities. Biomass, with its rich carbon feedstock, abundant availability, renewability, and versatile structures, has emerged as a promising precursor for porous carbon material synthesis. This review comprehensively summarizes the recent advances in biomass-derived porous carbon materials (BPCMs) encompassing synthetic strategy, morphology, structural composition, and multiple applications. We first review synthetic approaches aiming at regulating porosity, followed by morphological and composition features of BPCMs, with a special emphasis on elucidating the dimensional clarification and heteroatom doping effects. The discussion then extends to the wide-ranging applications of BPCMs, covering energy-related applications and CO₂ adsorption to environmental remediation. Finally, the review outlines the existing challenges and prospects in the field. In summary, this review systematically describes BPCMs and provides valuable guidance for researchers to select and synthesize BPCMs that meet specific functional requirements.

Key words: Biomass, Porous carbon, Pyrolysis, Heteroatom-doping, Supercapacitor, CO₂ adsorption

ZHAI Ziqi, LU Yumiao, LIU Guangyong, DING Wei-Lu, CAO Bobo, HE Hongyan. Recent Advances in Biomass-derived Porous Carbon Materials: Synthesis, Composition and Applications[J]. 高等学校化学研究, 2024, 40(1): 3-19.

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Recent Advances in Biomass-derived Porous Carbon Materials: Synthesis, Composition and Applications

Recent Advances in Biomass-derived Porous Carbon Materials: Synthesis, Composition and Applications

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