Graphdiyne Hybrid Nanowall Arrays for High-capacity Aqueous Rechargeable Zinc Ion Battery

doi:10.1007/s40242-021-1333-x

高等学校化学研究 ›› 2021, Vol. 37 ›› Issue (6): 1301-1308.doi: 10.1007/s40242-021-1333-x

Graphdiyne Hybrid Nanowall Arrays for High-capacity Aqueous Rechargeable Zinc Ion Battery

LI Jiaofu^1,2, CHEN Yanhuan^1,2, WANG Fuhui^1,2, GUO Jie^1,2, HE Feng¹, LIU Huibiao^1,2

1. CAS Key Laboratory of Organic Solids, Beijing National Laboratory for Molecular Sciences(BNLMS), CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;
2. University of Chinese Academy of Sciences, Beijing 100049, P. R. China

收稿日期:2021-08-24 修回日期:2021-09-21 出版日期:2021-11-23 发布日期:2021-11-23
通讯作者: LIU Huibiao E-mail:liuhb@iccas.ac.cn
基金资助:
This work was supported by the National Key Research and Development Project of China(No.2016YFA0200104), the National Natural Science Foundation of China(Nos.21875258, 21790050, 21790053) and the Key Program of the Chinese Academy of Sciences(No.QYZDY-SSWSLH015).

Graphdiyne Hybrid Nanowall Arrays for High-capacity Aqueous Rechargeable Zinc Ion Battery

LI Jiaofu^1,2, CHEN Yanhuan^1,2, WANG Fuhui^1,2, GUO Jie^1,2, HE Feng¹, LIU Huibiao^1,2

1. CAS Key Laboratory of Organic Solids, Beijing National Laboratory for Molecular Sciences(BNLMS), CAS Research/Education Center for Excellence in Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China;
2. University of Chinese Academy of Sciences, Beijing 100049, P. R. China

Received:2021-08-24 Revised:2021-09-21 Online:2021-11-23 Published:2021-11-23
Contact: LIU Huibiao E-mail:liuhb@iccas.ac.cn
Supported by:
This work was supported by the National Key Research and Development Project of China(No.2016YFA0200104), the National Natural Science Foundation of China(Nos.21875258, 21790050, 21790053) and the Key Program of the Chinese Academy of Sciences(No.QYZDY-SSWSLH015).

摘要/Abstract

摘要： Development of aqueous rechargeable zinc ion battery is an important direction towards grid energy storage sought in various applications. At present, the efficient utilization of aqueous rechargeable zinc ion batteries has been seriously affected due to the defects nature of the cathode materials, such as poor capacity, limited rate performance, and limited cycle stability. Therefore, the search for high-performance cathode materials is a main challenge in this field. Herein, we in-situ prepared graphdiyne-wrapped K_0.25·MnO₂(K_0.25·MnO₂@GDY) hybrid nanowall arrays as the cathode of aqueous rechargeable zinc ion battery. The hybridnanowall arrays have obviously alleviated the pulverization and sluggish kinetic process of MnO₂ cathode materials and shown high specific capacity(520 mA·h/g at a current density of 55 mA/g), which is near-full two-electron capacity. The high specific capacity was resulted from more than one Zn²⁺ (de)intercalation process occurring per formula unit, in which we observed a structural evolution that partially stemmed from ion exchange between the intercalated K⁺ and Zn²⁺ ions during the discharge process. The present investigation not only provides a new material for the aqueous rechargeable Zn ion batteries, also contributes a novel route for the development of next generation aqueous rechargeable Zn ion batteries with high capacity.

关键词: Graphdiyne, 2D material, Zinc ion battery, High-capacity, Energy storage

Abstract: Development of aqueous rechargeable zinc ion battery is an important direction towards grid energy storage sought in various applications. At present, the efficient utilization of aqueous rechargeable zinc ion batteries has been seriously affected due to the defects nature of the cathode materials, such as poor capacity, limited rate performance, and limited cycle stability. Therefore, the search for high-performance cathode materials is a main challenge in this field. Herein, we in-situ prepared graphdiyne-wrapped K_0.25·MnO₂(K_0.25·MnO₂@GDY) hybrid nanowall arrays as the cathode of aqueous rechargeable zinc ion battery. The hybridnanowall arrays have obviously alleviated the pulverization and sluggish kinetic process of MnO₂ cathode materials and shown high specific capacity(520 mA·h/g at a current density of 55 mA/g), which is near-full two-electron capacity. The high specific capacity was resulted from more than one Zn²⁺ (de)intercalation process occurring per formula unit, in which we observed a structural evolution that partially stemmed from ion exchange between the intercalated K⁺ and Zn²⁺ ions during the discharge process. The present investigation not only provides a new material for the aqueous rechargeable Zn ion batteries, also contributes a novel route for the development of next generation aqueous rechargeable Zn ion batteries with high capacity.

Key words: Graphdiyne, 2D material, Zinc ion battery, High-capacity, Energy storage

LI Jiaofu, CHEN Yanhuan, WANG Fuhui, GUO Jie, HE Feng, LIU Huibiao. Graphdiyne Hybrid Nanowall Arrays for High-capacity Aqueous Rechargeable Zinc Ion Battery[J]. 高等学校化学研究, 2021, 37(6): 1301-1308.

LI Jiaofu, CHEN Yanhuan, WANG Fuhui, GUO Jie, HE Feng, LIU Huibiao. Graphdiyne Hybrid Nanowall Arrays for High-capacity Aqueous Rechargeable Zinc Ion Battery[J]. Chemical Research in Chinese Universities, 2021, 37(6): 1301-1308.

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Graphdiyne Hybrid Nanowall Arrays for High-capacity Aqueous Rechargeable Zinc Ion Battery

Graphdiyne Hybrid Nanowall Arrays for High-capacity Aqueous Rechargeable Zinc Ion Battery

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