Diffusion Kinetics Study of Lithium Ion in the Graphdiyne Based Electrode

doi:10.1007/s40242-021-1316-y

高等学校化学研究 ›› 2021, Vol. 37 ›› Issue (6): 1289-1295.doi: 10.1007/s40242-021-1316-y

Diffusion Kinetics Study of Lithium Ion in the Graphdiyne Based Electrode

ZHANG Luwei, LIU Jingyi, BAI Ling, WANG Ning

Science Center for Material Creation and Energy Conversion, School of Chemistry and Chemical Engineering, Institute of Frontier and Interdisciplinary Science, Shandong University, Jinan 250100, P. R. China

收稿日期:2021-08-16 修回日期:2021-09-14 出版日期:2021-11-23 发布日期:2021-11-23
通讯作者: WANG Ning E-mail:wang_ning@sdu.edu.cn
基金资助:
This work was supported by the National Key Research and Development Project of China(No.2018YFA0703501), the National Natural Science Foundation of China(No.21875274), and the Young Scholarship Funding of Shandong University, China.

Diffusion Kinetics Study of Lithium Ion in the Graphdiyne Based Electrode

ZHANG Luwei, LIU Jingyi, BAI Ling, WANG Ning

Science Center for Material Creation and Energy Conversion, School of Chemistry and Chemical Engineering, Institute of Frontier and Interdisciplinary Science, Shandong University, Jinan 250100, P. R. China

Received:2021-08-16 Revised:2021-09-14 Online:2021-11-23 Published:2021-11-23
Contact: WANG Ning E-mail:wang_ning@sdu.edu.cn
Supported by:
This work was supported by the National Key Research and Development Project of China(No.2018YFA0703501), the National Natural Science Foundation of China(No.21875274), and the Young Scholarship Funding of Shandong University, China.

摘要/Abstract

摘要： Herein, we report a comparative investigation of the electrochemical lithium diffusion within graphidyne(GDY) based electrodes. The transfer kinetic behaviors of lithium ions during the insertion/extraction process are analyzed through different methods including the galvanostatic intermittent titration technique(GITT) and the electrochemical impedance spectroscopy (EIS). GDY with the morphology of nanosheets(GDY NS) shows lithium diffusion coefficients in the orders range of 10⁻¹²-10⁻¹³ cm²/s through the GITT method. Meanwhile, EIS indicates quite a lower value of lithium diffusion coefficients between 10⁻¹³ and 10⁻¹⁵ cm²/s, which indicates that the analysis technique has an influence on the evaluation of GDY-based electrodes. In addition, under the same measurement condition of GITT, GDY nanoparticles(GDY NP) exhibit a lower value of Li⁺ diffusion coefficient(10^-14-10^-16 cm²/s) during the charge-discharge process compared to those of GDY NS, which can be ascribed to the wide distributing range of particle size in GDY NP based electrodes. The analysis results in this work reveal that the aggregating forms of GDY electrode material have an important effect on the diffusion process of lithium ions, which provides a pathway to optimize the performance of GDY-based energy storage devices.

关键词: Graphdiyne, Diffusion kinetics, Lithium-ion battery, Electrode, Lithium diffusion coefficient

Abstract: Herein, we report a comparative investigation of the electrochemical lithium diffusion within graphidyne(GDY) based electrodes. The transfer kinetic behaviors of lithium ions during the insertion/extraction process are analyzed through different methods including the galvanostatic intermittent titration technique(GITT) and the electrochemical impedance spectroscopy (EIS). GDY with the morphology of nanosheets(GDY NS) shows lithium diffusion coefficients in the orders range of 10⁻¹²-10⁻¹³ cm²/s through the GITT method. Meanwhile, EIS indicates quite a lower value of lithium diffusion coefficients between 10⁻¹³ and 10⁻¹⁵ cm²/s, which indicates that the analysis technique has an influence on the evaluation of GDY-based electrodes. In addition, under the same measurement condition of GITT, GDY nanoparticles(GDY NP) exhibit a lower value of Li⁺ diffusion coefficient(10^-14-10^-16 cm²/s) during the charge-discharge process compared to those of GDY NS, which can be ascribed to the wide distributing range of particle size in GDY NP based electrodes. The analysis results in this work reveal that the aggregating forms of GDY electrode material have an important effect on the diffusion process of lithium ions, which provides a pathway to optimize the performance of GDY-based energy storage devices.

Key words: Graphdiyne, Diffusion kinetics, Lithium-ion battery, Electrode, Lithium diffusion coefficient

ZHANG Luwei, LIU Jingyi, BAI Ling, WANG Ning. Diffusion Kinetics Study of Lithium Ion in the Graphdiyne Based Electrode[J]. 高等学校化学研究, 2021, 37(6): 1289-1295.

ZHANG Luwei, LIU Jingyi, BAI Ling, WANG Ning. Diffusion Kinetics Study of Lithium Ion in the Graphdiyne Based Electrode[J]. Chemical Research in Chinese Universities, 2021, 37(6): 1289-1295.

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Diffusion Kinetics Study of Lithium Ion in the Graphdiyne Based Electrode

Diffusion Kinetics Study of Lithium Ion in the Graphdiyne Based Electrode

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