Covalent Organic Frameworks with trans-Dimensionally Vinylene-linked π-Conjugated Motifs

doi:10.1007/s40242-022-2010-4

高等学校化学研究 ›› 2022, Vol. 38 ›› Issue (2): 382-395.doi: 10.1007/s40242-022-2010-4

Covalent Organic Frameworks with trans-Dimensionally Vinylene-linked π-Conjugated Motifs

BI Shuai, MENG Fancheng, ZHANG Zixing, WU Dongqing, ZHANG Fan

School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, P. R. China

收稿日期:2022-01-05 修回日期:2022-02-16 出版日期:2022-04-01 发布日期:2022-05-18
通讯作者: ZHANG Fan E-mail:fan-zhang@sjtu.edu.cn
基金资助:
This work was supported by the National Natural Science Foundation of China (Nos.22005189, 21774072, 22075178), the China Postdoctoral Science Foundation(No.2020M681277), and the Science and Technology Commission of Shanghai Municipality, China(No.20JC1414900).

Covalent Organic Frameworks with trans-Dimensionally Vinylene-linked π-Conjugated Motifs

BI Shuai, MENG Fancheng, ZHANG Zixing, WU Dongqing, ZHANG Fan

School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, P. R. China

Received:2022-01-05 Revised:2022-02-16 Online:2022-04-01 Published:2022-05-18
Contact: ZHANG Fan E-mail:fan-zhang@sjtu.edu.cn
Supported by:
This work was supported by the National Natural Science Foundation of China (Nos.22005189, 21774072, 22075178), the China Postdoctoral Science Foundation(No.2020M681277), and the Science and Technology Commission of Shanghai Municipality, China(No.20JC1414900).

摘要/Abstract

摘要： Vinylene-linked covalent organic frameworks(COFs) are a class of promising porous organic materials that feature fully π-conjugated structures, high crystallinity, permanent porosity, ultrahigh chemical stability, and extraordinary optoelectronic properties. Over the past 5 years, this kind of material has been witnessed rapid development either in chemical synthesis or in potential applications. In this review, we summarize the chemistry to synthesize vinylene-linked COFs, especially the synthetic strategies involving activation of aryl methyl groups for condensation reaction. We then scrutinize the state-of-the-art development in properties and functions of this kind of COFs. Our own opinions on the further development of the vinylene-linked COFs are also presented for discussion.

关键词: Covalent organic framework(COF), Vinylene linkage, Stability, π-Conjugated structure, Semiconducting property

Abstract: Vinylene-linked covalent organic frameworks(COFs) are a class of promising porous organic materials that feature fully π-conjugated structures, high crystallinity, permanent porosity, ultrahigh chemical stability, and extraordinary optoelectronic properties. Over the past 5 years, this kind of material has been witnessed rapid development either in chemical synthesis or in potential applications. In this review, we summarize the chemistry to synthesize vinylene-linked COFs, especially the synthetic strategies involving activation of aryl methyl groups for condensation reaction. We then scrutinize the state-of-the-art development in properties and functions of this kind of COFs. Our own opinions on the further development of the vinylene-linked COFs are also presented for discussion.

Key words: Covalent organic framework(COF), Vinylene linkage, Stability, π-Conjugated structure, Semiconducting property

BI Shuai, MENG Fancheng, ZHANG Zixing, WU Dongqing, ZHANG Fan. Covalent Organic Frameworks with trans-Dimensionally Vinylene-linked π-Conjugated Motifs[J]. 高等学校化学研究, 2022, 38(2): 382-395.

BI Shuai, MENG Fancheng, ZHANG Zixing, WU Dongqing, ZHANG Fan. Covalent Organic Frameworks with trans-Dimensionally Vinylene-linked π-Conjugated Motifs[J]. Chemical Research in Chinese Universities, 2022, 38(2): 382-395.

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Covalent Organic Frameworks with trans-Dimensionally Vinylene-linked π-Conjugated Motifs

Covalent Organic Frameworks with trans-Dimensionally Vinylene-linked π-Conjugated Motifs

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