Two New Cadmium Metal-organic Frameworks Based on a Mixed-donor Ligand

doi:10.1007/s40242-016-5489-8

高等学校化学研究 ›› 2016, Vol. 32 ›› Issue (4): 539-544.doi: 10.1007/s40242-016-5489-8

Two New Cadmium Metal-organic Frameworks Based on a Mixed-donor Ligand

WANG Xiaofang, SONG Qingshan, PAN Ying, QIU Shilun, XUE Ming

State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, P. R. China

收稿日期:2015-12-16 修回日期:2016-02-26 出版日期:2016-08-01 发布日期:2016-04-11
通讯作者: XUE Ming E-mail:xueming@jlu.edu.cn
基金资助:
Supported by the National Natural Science Foundation of China(No.21571076).

Two New Cadmium Metal-organic Frameworks Based on a Mixed-donor Ligand

WANG Xiaofang, SONG Qingshan, PAN Ying, QIU Shilun, XUE Ming

State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, Jilin University, Changchun 130012, P. R. China

Received:2015-12-16 Revised:2016-02-26 Online:2016-08-01 Published:2016-04-11
Contact: XUE Ming E-mail:xueming@jlu.edu.cn
Supported by:
Supported by the National Natural Science Foundation of China(No.21571076).

摘要/Abstract

摘要：

The self-assembly of a prominent mixed-donor ligand, 5-[4-(1H-tetrazolyl)phen]isophthalic acid(H₃TZPI), with a Cd²⁺ center generates two new metal-organic frameworks:[Cd(H₂TZPI)₂(H₂O)₂]_n(JUC-163) and[Cd₂(TZPI)(μ₃-OH)(H₂O)₂]·H₂O·DMF(JUC-164). The two complexes demonstrate different structures for the ligand’s different coordination modes and configurations. JUC-163 shows a 2D layer structure and further forms into a 3D supramolecular framework by noncovalent interactions(C-H…O, O-H…N and π…π interactions), whereas JUC-164 exhibits a fascinating 3D framework for the outstanding coordination modes and configurations of the ligand, which are fit for the complex structure. And also, the factor of different cadmium salts(chloride and nitrate) which are used in synthesis progress is worth to notice for the construction of the two distinct structures. The luminescent properties of these metal-organic frameworks were also investigated.

关键词: Cadmium, Mixed-donor ligand, Metal-organic framework, Luminescence

Abstract:

Key words: Cadmium, Mixed-donor ligand, Metal-organic framework, Luminescence

WANG Xiaofang, SONG Qingshan, PAN Ying, QIU Shilun, XUE Ming. Two New Cadmium Metal-organic Frameworks Based on a Mixed-donor Ligand[J]. 高等学校化学研究, 2016, 32(4): 539-544.

WANG Xiaofang, SONG Qingshan, PAN Ying, QIU Shilun, XUE Ming. Two New Cadmium Metal-organic Frameworks Based on a Mixed-donor Ligand[J]. Chemical Research in Chinese Universities, 2016, 32(4): 539-544.

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Two New Cadmium Metal-organic Frameworks Based on a Mixed-donor Ligand

Two New Cadmium Metal-organic Frameworks Based on a Mixed-donor Ligand

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