Recent Advances in CO2 Reduction Reaction to Value-added C1 Products by Single-atom Catalysts

doi:10.1007/s40242-023-3001-9

高等学校化学研究 ›› 2023, Vol. 39 ›› Issue (4): 527-544.doi: 10.1007/s40242-023-3001-9

Recent Advances in CO₂ Reduction Reaction to Value-added C1 Products by Single-atom Catalysts

LI Boyang¹, OU Honghui², CHEN Shenghua^1,2, SU Ya-Qiong¹, WANG Dingsheng²

1. School of Chemistry, National Innovation Platform(Center) for IndustryEducation Integration of Energy Storage Technology, Xi'an Key Laboratory of Sustainable Energy Materials Chemistry, State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an 710049, P.R. China;
2. Engineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P.R. China

收稿日期:2023-01-02 出版日期:2023-08-01 发布日期:2023-07-18
通讯作者: CHEN Shenghua, SU Ya-Qiong, WANG Dingsheng E-mail:shenghchen@163.com;yqsu1989@xjtu.edu.cn;wangdingsheng@mail.tsinghua.edu.cn
基金资助:
This work was supported by the National Key R&D Program of China(No. 2018YFA0702003), the National Natural Science Foundation of China(Nos. 21890383, 22171157, and 52002249), the "Young Talent Support Plan" of Xi'an Jiaotong University, China and the Open Funds of State Key Laboratory of Physical Chemistry of Solid Surfaces of Xiamen University, China(No.202018).

Recent Advances in CO₂ Reduction Reaction to Value-added C1 Products by Single-atom Catalysts

LI Boyang¹, OU Honghui², CHEN Shenghua^1,2, SU Ya-Qiong¹, WANG Dingsheng²

1. School of Chemistry, National Innovation Platform(Center) for IndustryEducation Integration of Energy Storage Technology, Xi'an Key Laboratory of Sustainable Energy Materials Chemistry, State Key Laboratory of Electrical Insulation and Power Equipment, Xi'an Jiaotong University, Xi'an 710049, P.R. China;
2. Engineering Research Center of Advanced Rare Earth Materials, Department of Chemistry, Tsinghua University, Beijing 100084, P.R. China

Received:2023-01-02 Online:2023-08-01 Published:2023-07-18
Contact: CHEN Shenghua, SU Ya-Qiong, WANG Dingsheng E-mail:shenghchen@163.com;yqsu1989@xjtu.edu.cn;wangdingsheng@mail.tsinghua.edu.cn
Supported by:
This work was supported by the National Key R&D Program of China(No. 2018YFA0702003), the National Natural Science Foundation of China(Nos. 21890383, 22171157, and 52002249), the "Young Talent Support Plan" of Xi'an Jiaotong University, China and the Open Funds of State Key Laboratory of Physical Chemistry of Solid Surfaces of Xiamen University, China(No.202018).

摘要/Abstract

摘要： The CO₂reduction reaction driven by sustainable electrical energy to value-added hydrocarbons is highly attractive because it can address both energy and environmental issues. The precise and rational development of corresponding electrocatalysts is of great importance to these kinds of reactions. Single-atom catalysts with unique electronic structures and coordination environments have become promising candidates, which may offer enhanced electrocatalytic performance. Herein, we summarize the recent development in the efficient fabrication of single-atom catalysts and their further application in CO₂ reduction. The various strategies for SACs preparation and characterization methods are highlighted to give a comprehensive understanding of the relationship between metal active sites and catalytic ability. The reaction mechanisms of electronic CO₂ reduction over single-atom catalysts are elaborated. Finally, the challenges and perspectives for the implementation of single-atom catalysts in CO₂ reduction are discussed.

关键词: CO₂ reduction, Single-atom catalyst, Electrocatalysis

Abstract: The CO₂reduction reaction driven by sustainable electrical energy to value-added hydrocarbons is highly attractive because it can address both energy and environmental issues. The precise and rational development of corresponding electrocatalysts is of great importance to these kinds of reactions. Single-atom catalysts with unique electronic structures and coordination environments have become promising candidates, which may offer enhanced electrocatalytic performance. Herein, we summarize the recent development in the efficient fabrication of single-atom catalysts and their further application in CO₂ reduction. The various strategies for SACs preparation and characterization methods are highlighted to give a comprehensive understanding of the relationship between metal active sites and catalytic ability. The reaction mechanisms of electronic CO₂ reduction over single-atom catalysts are elaborated. Finally, the challenges and perspectives for the implementation of single-atom catalysts in CO₂ reduction are discussed.

Key words: CO₂ reduction, Single-atom catalyst, Electrocatalysis

LI Boyang, OU Honghui, CHEN Shenghua, SU Ya-Qiong, WANG Dingsheng. Recent Advances in CO₂ Reduction Reaction to Value-added C1 Products by Single-atom Catalysts[J]. 高等学校化学研究, 2023, 39(4): 527-544.

LI Boyang, OU Honghui, CHEN Shenghua, SU Ya-Qiong, WANG Dingsheng. Recent Advances in CO₂ Reduction Reaction to Value-added C1 Products by Single-atom Catalysts[J]. Chemical Research in Chinese Universities, 2023, 39(4): 527-544.

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Recent Advances in CO₂ Reduction Reaction to Value-added C1 Products by Single-atom Catalysts

Recent Advances in CO₂ Reduction Reaction to Value-added C1 Products by Single-atom Catalysts

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