Recent Advances in Mechanism of AIE Mechanochromic Materials

doi:10.1007/s40242-021-0431-0

高等学校化学研究 ›› 2021, Vol. 37 ›› Issue (1): 100-109.doi: 10.1007/s40242-021-0431-0

Recent Advances in Mechanism of AIE Mechanochromic Materials

WANG Lipeng, LIU Leijing, XU Bin, TIAN Wenjing

State Key Laboratory of Supramolecular Structure and Materials, Jilin University, Changchun 130012, P. R. China

收稿日期:2020-12-19 修回日期:2021-01-11 出版日期:2021-02-01 发布日期:2021-02-03
通讯作者: LIU Leijing, TIAN Wenjing E-mail:liuleijing@jlu.edu.cn;wjtian@jlu.edu.cn
基金资助:
This work is supported by the National Natural Science Foundation of China(Nos. 21835001, 52073116, 51773080).

Recent Advances in Mechanism of AIE Mechanochromic Materials

WANG Lipeng, LIU Leijing, XU Bin, TIAN Wenjing

State Key Laboratory of Supramolecular Structure and Materials, Jilin University, Changchun 130012, P. R. China

Received:2020-12-19 Revised:2021-01-11 Online:2021-02-01 Published:2021-02-03
Contact: LIU Leijing, TIAN Wenjing E-mail:liuleijing@jlu.edu.cn;wjtian@jlu.edu.cn
Supported by:
This work is supported by the National Natural Science Foundation of China(Nos. 21835001, 52073116, 51773080).

摘要/Abstract

摘要： Organic mechanochromic materials(also known as piezochromic materials), whose color or emission changes under mechanical force, have attracted great interest owing to their potential applications in pressure sensors, rewritable materials, optical storage, and security ink. Organic mechanochromic materials with aggregation-induced emission(AIE) features have better deve-lopment prospects and research value owing to their excellent optical properties. To date, mechanochromism has mostly been realized by means of mechanical grinding. Nevertheless, the magnitude of the grinding force is usually uncontrollable and its direction is anisotropic, making it awkward to study the mechanism of mechanochromic materials. On the contrary, hydrostatic pressure, whose magnitude and direction are controllable, is a more valid and go-vernable method to investigate the mechanism of mechanochromic materials, which can help us to construct a meaningful structure-property relationship and understand the latent origin of the me-chanochromism. Furthermore, it is conducive to developing other mechanochromic material systems with desired chemical and phy-sical properties. In this review, we focus on the recent progress in the mechanism of organic mechanochromic materials with AIE features under hydrostatic pressure. Four types of mechanisms are included:intermolecular interaction change, intramolecular conformation change, transformation from locally excited state to intramolecular charge-transfer state, and intra- and inter-molecular effects induced by hydrostatic pressure, respectively.

关键词: Aggregation-induced emission, Mechanism, Mechanochromic, Hydrostatic pressure

Abstract: Organic mechanochromic materials(also known as piezochromic materials), whose color or emission changes under mechanical force, have attracted great interest owing to their potential applications in pressure sensors, rewritable materials, optical storage, and security ink. Organic mechanochromic materials with aggregation-induced emission(AIE) features have better deve-lopment prospects and research value owing to their excellent optical properties. To date, mechanochromism has mostly been realized by means of mechanical grinding. Nevertheless, the magnitude of the grinding force is usually uncontrollable and its direction is anisotropic, making it awkward to study the mechanism of mechanochromic materials. On the contrary, hydrostatic pressure, whose magnitude and direction are controllable, is a more valid and go-vernable method to investigate the mechanism of mechanochromic materials, which can help us to construct a meaningful structure-property relationship and understand the latent origin of the me-chanochromism. Furthermore, it is conducive to developing other mechanochromic material systems with desired chemical and phy-sical properties. In this review, we focus on the recent progress in the mechanism of organic mechanochromic materials with AIE features under hydrostatic pressure. Four types of mechanisms are included:intermolecular interaction change, intramolecular conformation change, transformation from locally excited state to intramolecular charge-transfer state, and intra- and inter-molecular effects induced by hydrostatic pressure, respectively.

Key words: Aggregation-induced emission, Mechanism, Mechanochromic, Hydrostatic pressure

WANG Lipeng, LIU Leijing, XU Bin, TIAN Wenjing. Recent Advances in Mechanism of AIE Mechanochromic Materials[J]. 高等学校化学研究, 2021, 37(1): 100-109.

WANG Lipeng, LIU Leijing, XU Bin, TIAN Wenjing. Recent Advances in Mechanism of AIE Mechanochromic Materials[J]. Chemical Research in Chinese Universities, 2021, 37(1): 100-109.

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Recent Advances in Mechanism of AIE Mechanochromic Materials

Recent Advances in Mechanism of AIE Mechanochromic Materials

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