Reconfigurable Plasmonic Nanostructures Controlled by DNA Origami

doi:10.1007/s40242-020-9078-5

高等学校化学研究 ›› 2020, Vol. 36 ›› Issue (2): 296-300.doi: 10.1007/s40242-020-9078-5

Reconfigurable Plasmonic Nanostructures Controlled by DNA Origami

LONG Qipeng, YU Hanyang, LI Zhe

Department of Biomedical Engineering, College of Engineering and Applied Sciences, Nanjing University, Nanjing 210093, P. R. China

收稿日期:2019-12-02 修回日期:2019-12-25 出版日期:2020-04-01 发布日期:2020-01-13
通讯作者: YU Hanyang, LI Zhe E-mail:zheli@nju.edu.cn;hanyangyu@nju.edu.cn
基金资助:
Supported by the National Key Research and Development Program of China(No.2016YFA0502600) and the National Natural Science Foundation of China(Nos.21603100, 21708018).

Reconfigurable Plasmonic Nanostructures Controlled by DNA Origami

LONG Qipeng, YU Hanyang, LI Zhe

Department of Biomedical Engineering, College of Engineering and Applied Sciences, Nanjing University, Nanjing 210093, P. R. China

Received:2019-12-02 Revised:2019-12-25 Online:2020-04-01 Published:2020-01-13
Contact: YU Hanyang, LI Zhe E-mail:zheli@nju.edu.cn;hanyangyu@nju.edu.cn
Supported by:
Supported by the National Key Research and Development Program of China(No.2016YFA0502600) and the National Natural Science Foundation of China(Nos.21603100, 21708018).

摘要/Abstract

摘要： Precise surface functionalization and reconfigurable capability of nanomaterials are essential to construct complex nanostructures with specific functions. Here we show the assembly of a reconfigurable plasmonic nanostructure, which executes both conformational and plasmonic changes in response to DNA strands. In this work, different sized gold nanoparticles(AuNPs) were arranged site-specifically on the surface of a DNA origami clamp nanostructure. The opening and closing of the DNA origami clamp could be precisely controlled by a series of strand displacement reactions. Therefore, the patterns of these AuNPs could be switched between two different configurations. The observed plasmon band shift indicates the change of the plasmonic interactions among the assembled AuNPs. Our study achieves the construction of reconfigurable nanomaterials with tunable plasmonic interactions, and will enrich the toolbox of DNA-based functional nanomachinery.

关键词: DNA origami, Gold nanoparticle, Reconfigurable nanostructure, Plasmonic nanostructure

Abstract: Precise surface functionalization and reconfigurable capability of nanomaterials are essential to construct complex nanostructures with specific functions. Here we show the assembly of a reconfigurable plasmonic nanostructure, which executes both conformational and plasmonic changes in response to DNA strands. In this work, different sized gold nanoparticles(AuNPs) were arranged site-specifically on the surface of a DNA origami clamp nanostructure. The opening and closing of the DNA origami clamp could be precisely controlled by a series of strand displacement reactions. Therefore, the patterns of these AuNPs could be switched between two different configurations. The observed plasmon band shift indicates the change of the plasmonic interactions among the assembled AuNPs. Our study achieves the construction of reconfigurable nanomaterials with tunable plasmonic interactions, and will enrich the toolbox of DNA-based functional nanomachinery.

Key words: DNA origami, Gold nanoparticle, Reconfigurable nanostructure, Plasmonic nanostructure

LONG Qipeng, YU Hanyang, LI Zhe. Reconfigurable Plasmonic Nanostructures Controlled by DNA Origami[J]. 高等学校化学研究, 2020, 36(2): 296-300.

LONG Qipeng, YU Hanyang, LI Zhe. Reconfigurable Plasmonic Nanostructures Controlled by DNA Origami[J]. Chemical Research in Chinese Universities, 2020, 36(2): 296-300.

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Reconfigurable Plasmonic Nanostructures Controlled by DNA Origami

Reconfigurable Plasmonic Nanostructures Controlled by DNA Origami

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