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高等学校化学研究 ›› 2024, Vol. 40 ›› Issue (6): 943-963.doi: 10.1007/s40242-024-4179-1

• Review • 上一篇    下一篇

Synthesis and Utilization of MXene/MOF Hybrid Composite Materials

JI Houqiang1, LIU Yuxin2, DU Guangyu2, HUANG Tianyu1, ZHU Ying1, SUN Yangyang1, PANG Huan1   

  1. 1. School of Chemistry and Chemical Engineering (Institute for Innovative Materials and Energy), Yangzhou University, Yangzhou 225009, P. R. China;
    2. Department of Applied Physics, The Hong Kong Polytechnic University, Hung Hom, Kowloon, 999077, Hong Kong, P. R. China
  • 收稿日期:2024-08-14 出版日期:2024-12-01 发布日期:2024-10-26
  • 通讯作者: PANG Huan,panghuan@yzu.edu.cn;SUN Yangyang,yangyangsun@yzu.edu.cn E-mail:panghuan@yzu.edu.cn;yangyangsun@yzu.edu.cn
  • 基金资助:
    This work was supported by the National Natural Science Foundation of China (No. 52371240), and the Jiangsu Province Excellent Postdoctoral Program, China (No. 2022ZB613).

Synthesis and Utilization of MXene/MOF Hybrid Composite Materials

JI Houqiang1, LIU Yuxin2, DU Guangyu2, HUANG Tianyu1, ZHU Ying1, SUN Yangyang1, PANG Huan1   

  1. 1. School of Chemistry and Chemical Engineering (Institute for Innovative Materials and Energy), Yangzhou University, Yangzhou 225009, P. R. China;
    2. Department of Applied Physics, The Hong Kong Polytechnic University, Hung Hom, Kowloon, 999077, Hong Kong, P. R. China
  • Received:2024-08-14 Online:2024-12-01 Published:2024-10-26
  • Contact: PANG Huan,panghuan@yzu.edu.cn;SUN Yangyang,yangyangsun@yzu.edu.cn E-mail:panghuan@yzu.edu.cn;yangyangsun@yzu.edu.cn
  • Supported by:
    This work was supported by the National Natural Science Foundation of China (No. 52371240), and the Jiangsu Province Excellent Postdoctoral Program, China (No. 2022ZB613).

摘要: Metal-organic frameworks (MOFs) are crystalline porous architectures formed by the coordination of organic ligands with metal ions or clusters. MOFs are notable for their vast surface area, abundant active sites, high porosity, and tunable properties. However, their application in energy storage and catalysis is impeded by limited conductivity and chemical stability. A promising approach to mitigating these constraints is the integration of MOFs with other functional or conductive materials. MXenes, with their distinctive layered structure, exceptional electrical conductivity, and rich surface functional groups, provide numerous advantages when combined with MOFs. This review encapsulates the synthesis methodologies of MXene/MOF composites and explores their applications across various domains, including lithium-ion batteries, supercapacitors, lithium-sulfur batteries, zinc-ion batteries, electrocatalysts, and photocatalysts.

关键词: MXene/MOF hybrid, Battery, Supercapacitor, Electrocatalyst, Photocatalyst

Abstract: Metal-organic frameworks (MOFs) are crystalline porous architectures formed by the coordination of organic ligands with metal ions or clusters. MOFs are notable for their vast surface area, abundant active sites, high porosity, and tunable properties. However, their application in energy storage and catalysis is impeded by limited conductivity and chemical stability. A promising approach to mitigating these constraints is the integration of MOFs with other functional or conductive materials. MXenes, with their distinctive layered structure, exceptional electrical conductivity, and rich surface functional groups, provide numerous advantages when combined with MOFs. This review encapsulates the synthesis methodologies of MXene/MOF composites and explores their applications across various domains, including lithium-ion batteries, supercapacitors, lithium-sulfur batteries, zinc-ion batteries, electrocatalysts, and photocatalysts.

Key words: MXene/MOF hybrid, Battery, Supercapacitor, Electrocatalyst, Photocatalyst