Tuning Photodetection Band of MAPbX3(X=Cl/Br/I) Perovskite Single Crystals by Sub-nano Carbon Dot Doping

doi:10.1007/s40242-023-3086-1

高等学校化学研究 ›› 2023, Vol. 39 ›› Issue (4): 654-659.doi: 10.1007/s40242-023-3086-1

Tuning Photodetection Band of MAPbX₃(X=Cl/Br/I) Perovskite Single Crystals by Sub-nano Carbon Dot Doping

ZHU Xia¹, AN Jiakun¹, CHEN Gaoyu¹, XING Chenyu¹, BAO Jianchun¹, XU Xiangxing^1,2

1. School of Chemistry and Materials Science, Nanjing Normal University, Nanjing 210023, P.R. China;
2. State Key Laboratory of Coordination Chemistry, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210093, P.R. China

收稿日期:2023-04-04 出版日期:2023-08-01 发布日期:2023-07-18
通讯作者: BAO Jianchun, XU Xiangxing E-mail:baojianchun@njnu.edu.cn;xuxx@njnu.edu.cn
基金资助:
This work was supported by the the National Natural Science Foundation of China (No.22175095).

Tuning Photodetection Band of MAPbX₃(X=Cl/Br/I) Perovskite Single Crystals by Sub-nano Carbon Dot Doping

ZHU Xia¹, AN Jiakun¹, CHEN Gaoyu¹, XING Chenyu¹, BAO Jianchun¹, XU Xiangxing^1,2

1. School of Chemistry and Materials Science, Nanjing Normal University, Nanjing 210023, P.R. China;
2. State Key Laboratory of Coordination Chemistry, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210093, P.R. China

Received:2023-04-04 Online:2023-08-01 Published:2023-07-18
Contact: BAO Jianchun, XU Xiangxing E-mail:baojianchun@njnu.edu.cn;xuxx@njnu.edu.cn
Supported by:
This work was supported by the the National Natural Science Foundation of China (No.22175095).

摘要/Abstract

摘要： Perovskite single crystals are prominent semiconductor materials due to their high carrier mobility, long carrier diffusion length, and large absorption coefficient. They can be used as optoelectronic functional materials for narrowband or broadband photodetectors. In this report, the photodetection band tunability was achieved by doping MAPbX₃(MA=methylammonium, X=Cl/Br/I) perovskite single crystals with sub-nano carbon dots (MAPbX₃-C). The sub-nano size and good dispersibility of the carbon dots ensured controllable doping. The absorption of the sub-nano carbon dots and trap states in the MAPbX₃-C single crystals resulted in the special responsivity spectrum features.

关键词: Sub-nano, Carbon dot, Perovskite, Single crystal, Photodetector

Abstract: Perovskite single crystals are prominent semiconductor materials due to their high carrier mobility, long carrier diffusion length, and large absorption coefficient. They can be used as optoelectronic functional materials for narrowband or broadband photodetectors. In this report, the photodetection band tunability was achieved by doping MAPbX₃(MA=methylammonium, X=Cl/Br/I) perovskite single crystals with sub-nano carbon dots (MAPbX₃-C). The sub-nano size and good dispersibility of the carbon dots ensured controllable doping. The absorption of the sub-nano carbon dots and trap states in the MAPbX₃-C single crystals resulted in the special responsivity spectrum features.

Key words: Sub-nano, Carbon dot, Perovskite, Single crystal, Photodetector

ZHU Xia, AN Jiakun, CHEN Gaoyu, XING Chenyu, BAO Jianchun, XU Xiangxing. Tuning Photodetection Band of MAPbX₃(X=Cl/Br/I) Perovskite Single Crystals by Sub-nano Carbon Dot Doping[J]. 高等学校化学研究, 2023, 39(4): 654-659.

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Tuning Photodetection Band of MAPbX₃(X=Cl/Br/I) Perovskite Single Crystals by Sub-nano Carbon Dot Doping

Tuning Photodetection Band of MAPbX₃(X=Cl/Br/I) Perovskite Single Crystals by Sub-nano Carbon Dot Doping

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