Covalent Organic Frameworks Based Single-site Electrocatalysts for Oxygen Reduction Reaction

doi:10.1007/s40242-022-2219-2

高等学校化学研究 ›› 2022, Vol. 38 ›› Issue (5): 1151-1162.doi: 10.1007/s40242-022-2219-2

Covalent Organic Frameworks Based Single-site Electrocatalysts for Oxygen Reduction Reaction

BU Ran^1,2, LU Yingying^1,2, ZHANG Bing^1,2

1. State Key Laboratory of Chemical Engineering, Institute of Pharmaceutical Engineering, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, P. R. China;
2. ZJU-Hangzhou Global Scientific and Technological Innovation Center, Hangzhou 311200, P. R. China

收稿日期:2022-06-29 出版日期:2022-10-01 发布日期:2022-10-08
通讯作者: LU Yingying, ZHANG Bing E-mail:yingyinglu@zju.edu.cn;bzhang219@zju.edu.cn
基金资助:
This work was supported by the National Key R&D Program of China(No. 2018YFA0209600), the National Natural Science Foundation of China(Nos. 22022813, 21878268), the Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang Province, China(No.2019R01006), the National Postdoctoral Program for Innovative Talents, China(No.BX20180203), and the Project of the Chongqing Key Laboratory for Advanced Materials & Technologies of Clean Energies, China(No.JJNY202003).

Covalent Organic Frameworks Based Single-site Electrocatalysts for Oxygen Reduction Reaction

BU Ran^1,2, LU Yingying^1,2, ZHANG Bing^1,2

1. State Key Laboratory of Chemical Engineering, Institute of Pharmaceutical Engineering, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, P. R. China;
2. ZJU-Hangzhou Global Scientific and Technological Innovation Center, Hangzhou 311200, P. R. China

Received:2022-06-29 Online:2022-10-01 Published:2022-10-08
Contact: LU Yingying, ZHANG Bing E-mail:yingyinglu@zju.edu.cn;bzhang219@zju.edu.cn
Supported by:
This work was supported by the National Key R&D Program of China(No. 2018YFA0209600), the National Natural Science Foundation of China(Nos. 22022813, 21878268), the Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang Province, China(No.2019R01006), the National Postdoctoral Program for Innovative Talents, China(No.BX20180203), and the Project of the Chongqing Key Laboratory for Advanced Materials & Technologies of Clean Energies, China(No.JJNY202003).

摘要/Abstract

摘要： Single site catalysts(SSCs) are a new type of heterogeneous catalysts formed by isolated metal atoms supported on kinds of substrates. SSCs have shown great potential for energy conversion and storage in recent years, especially for oxygen reduction reactions(ORR). Typically, SSCs are confined on the substrate by strong chemical interactions, such as coordination bonds. Therefore, the surface chemical environment and porous properties of the supports are crucial to the performance of SSCs. In recent years, COFs have become excellent candidates for preparing SSCs as they can precisely assemble monomers into highly ordered crystalline porous materials with a fine structure and definite components. In this review, we not only summarize the characteristics and advantages of COFs based SSCs, but also highlight the applications of COFs constructed from different single active sites for ORR in recent years. Finally, challenges in practical application, feasible strategies and perspectives are proposed for the of COFs based SSCs.

关键词: Covalent organic framework, Oxygen reduction reaction, Single site catalyst, Energy conversion, Carbon-based catalyst

Abstract: Single site catalysts(SSCs) are a new type of heterogeneous catalysts formed by isolated metal atoms supported on kinds of substrates. SSCs have shown great potential for energy conversion and storage in recent years, especially for oxygen reduction reactions(ORR). Typically, SSCs are confined on the substrate by strong chemical interactions, such as coordination bonds. Therefore, the surface chemical environment and porous properties of the supports are crucial to the performance of SSCs. In recent years, COFs have become excellent candidates for preparing SSCs as they can precisely assemble monomers into highly ordered crystalline porous materials with a fine structure and definite components. In this review, we not only summarize the characteristics and advantages of COFs based SSCs, but also highlight the applications of COFs constructed from different single active sites for ORR in recent years. Finally, challenges in practical application, feasible strategies and perspectives are proposed for the of COFs based SSCs.

Key words: Covalent organic framework, Oxygen reduction reaction, Single site catalyst, Energy conversion, Carbon-based catalyst

BU Ran, LU Yingying, ZHANG Bing. Covalent Organic Frameworks Based Single-site Electrocatalysts for Oxygen Reduction Reaction[J]. 高等学校化学研究, 2022, 38(5): 1151-1162.

BU Ran, LU Yingying, ZHANG Bing. Covalent Organic Frameworks Based Single-site Electrocatalysts for Oxygen Reduction Reaction[J]. Chemical Research in Chinese Universities, 2022, 38(5): 1151-1162.

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Covalent Organic Frameworks Based Single-site Electrocatalysts for Oxygen Reduction Reaction

Covalent Organic Frameworks Based Single-site Electrocatalysts for Oxygen Reduction Reaction

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