Basic Catalytic Performance of Amino and Acylamide Functionalized Metal-organic Framework in the Synthesis of Chloropropene Carbonate from CO2 Under Atmospheric Pressure

doi:10.1007/s40242-016-6076-8

高等学校化学研究 ›› 2016, Vol. 32 ›› Issue (5): 838-842.doi: 10.1007/s40242-016-6076-8

Basic Catalytic Performance of Amino and Acylamide Functionalized Metal-organic Framework in the Synthesis of Chloropropene Carbonate from CO₂ Under Atmospheric Pressure

SONG Lili, CHEN Chao, CHEN Xiangbin, ZHANG Ning

Institute of Applied Chemistry, College of Chemistry, Nanchang University, Nanchang 330031, P. R. China

收稿日期:2016-03-04 修回日期:2016-05-26 出版日期:2016-10-01 发布日期:2016-06-20
通讯作者: CHEN Chao, ZHANG Ning E-mail:chaochen@ncu.edu.cn;nzhang.ncu@163.com
基金资助:
Supported by the National Natural Science Foundation of China(Nos.21261017, 21561020) and the Union of Industry Study Fund of Dongguan City, China(No.2014509112210).

Basic Catalytic Performance of Amino and Acylamide Functionalized Metal-organic Framework in the Synthesis of Chloropropene Carbonate from CO₂ Under Atmospheric Pressure

SONG Lili, CHEN Chao, CHEN Xiangbin, ZHANG Ning

Institute of Applied Chemistry, College of Chemistry, Nanchang University, Nanchang 330031, P. R. China

Received:2016-03-04 Revised:2016-05-26 Online:2016-10-01 Published:2016-06-20
Contact: CHEN Chao, ZHANG Ning E-mail:chaochen@ncu.edu.cn;nzhang.ncu@163.com
Supported by:
Supported by the National Natural Science Foundation of China(Nos.21261017, 21561020) and the Union of Industry Study Fund of Dongguan City, China(No.2014509112210).

摘要/Abstract

摘要：

In this work, a metal-organic framework with free standing basic groups(e. g., amino and acylamide groups) decorated in the pore wall was utilized to catalyze the CO₂ cycloaddition reaction and its basic properties were tested in Knoevenagel condensation reactions. The results reveal that the metal-organic framework(MOF) material has excellent catalytic activity and high repeatability for the synthesis of chloropropene carbonate from CO₂ and epichlorohydrin with no co-catalyst under mild reaction conditions, suggesting that it is a promising heteroge-neous catalyst for CO₂ cycloaddition reaction.

关键词: Metal-organic framework, Heterogeneous catalysis, CO₂, Chloropropene carbonate

Abstract:

Key words: Metal-organic framework, Heterogeneous catalysis, CO₂, Chloropropene carbonate

SONG Lili, CHEN Chao, CHEN Xiangbin, ZHANG Ning. Basic Catalytic Performance of Amino and Acylamide Functionalized Metal-organic Framework in the Synthesis of Chloropropene Carbonate from CO₂ Under Atmospheric Pressure[J]. 高等学校化学研究, 2016, 32(5): 838-842.

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Basic Catalytic Performance of Amino and Acylamide Functionalized Metal-organic Framework in the Synthesis of Chloropropene Carbonate from CO₂ Under Atmospheric Pressure

Basic Catalytic Performance of Amino and Acylamide Functionalized Metal-organic Framework in the Synthesis of Chloropropene Carbonate from CO₂ Under Atmospheric Pressure

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