Two-dimensional Metal-Organic Frameworks and Derivatives for Electrocatalysis

doi:10.1007/s40242-020-0163-6

摘要/Abstract

摘要： The most important topics in the world today are environmental and resource issues. The development of green and clean energy is still one of the great challenges of social sustainable development. Two-dimensional(2D) metal-organic frameworks(MOFs) and derivatives have exceptional potential as high-efficiency electrocatalysts for clean energy technologies. This review summarizes various synthesis strategies and applications of 2D MOFs and derivatives in electrocatalysis. Firstly, we will outline the advantages and uniqueness of 2D MOFs and derivatives, as well as their applicable areas. Secondly, the synthetic strategies of 2D MOFs and derivatives are briefly classified. Each category is summarized and we list classic representative fabrication methods, including specific fabrication methods and mechanisms, corresponding structural characteristics, and insights into the advantages and limitations of the synthesis method. Thirdly, we separately classify and summarize the application of 2D MOFs and derivatives in electrocatalysis, including electrocatalytic water splitting, oxygen reduction reaction(ORR), CO₂ reduction reaction(CO₂RR), and other electrocatalytic applications. Finally, the development prospects and existing challenges to 2D MOFs and derivatives are discussed.

关键词: Two-dimensional, Metal-organic framework, Derivative, Synthesis strategy, Electrocatalysis

Abstract: The most important topics in the world today are environmental and resource issues. The development of green and clean energy is still one of the great challenges of social sustainable development. Two-dimensional(2D) metal-organic frameworks(MOFs) and derivatives have exceptional potential as high-efficiency electrocatalysts for clean energy technologies. This review summarizes various synthesis strategies and applications of 2D MOFs and derivatives in electrocatalysis. Firstly, we will outline the advantages and uniqueness of 2D MOFs and derivatives, as well as their applicable areas. Secondly, the synthetic strategies of 2D MOFs and derivatives are briefly classified. Each category is summarized and we list classic representative fabrication methods, including specific fabrication methods and mechanisms, corresponding structural characteristics, and insights into the advantages and limitations of the synthesis method. Thirdly, we separately classify and summarize the application of 2D MOFs and derivatives in electrocatalysis, including electrocatalytic water splitting, oxygen reduction reaction(ORR), CO₂ reduction reaction(CO₂RR), and other electrocatalytic applications. Finally, the development prospects and existing challenges to 2D MOFs and derivatives are discussed.

Key words: Two-dimensional, Metal-organic framework, Derivative, Synthesis strategy, Electrocatalysis

WEN Jinguli, LI Yuwen, GAO Junkuo. Two-dimensional Metal-Organic Frameworks and Derivatives for Electrocatalysis[J]. 高等学校化学研究, 2020, 36(4): 662-679.

WEN Jinguli, LI Yuwen, GAO Junkuo. Two-dimensional Metal-Organic Frameworks and Derivatives for Electrocatalysis[J]. Chemical Research in Chinese Universities, 2020, 36(4): 662-679.

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