Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review

doi:10.1007/s40242-020-0103-5

高等学校化学研究 ›› 2020, Vol. 36 ›› Issue (3): 377-385.doi: 10.1007/s40242-020-0103-5

Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review

YUAN Hong^1,2, LIU Jia^2,3, LU Yang², ZHAO Chenzi², CHENG Xinbing², NAN Haoxiong⁴, LIU Quanbing⁴, HUANG Jiaqi¹, ZHANG Qiang²

1. Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, P. R. China;
2. Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, P. R. China;
3. Beijing Key Laboratory of Lignocellulosic Chemistry, Beijing Forestry University, Beijing 100083, P. R. China;
4. School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006, P. R. China

收稿日期:2020-04-11 修回日期:2020-05-01 出版日期:2020-06-01 发布日期:2020-05-30
通讯作者: ZHANG Qiang E-mail:zhang-qiang@mails.tsinghua.edu.cn
基金资助:
Supported by the National Natural Science Foundation of China(Nos.21808124, 21825501, U1801257), the National Key Research and Development Program of China(Nos.2016YFA0202500, 2016YFA0200102) and the China Postdoctoral Science Foundation(No.2019T120098).

Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review

YUAN Hong^1,2, LIU Jia^2,3, LU Yang², ZHAO Chenzi², CHENG Xinbing², NAN Haoxiong⁴, LIU Quanbing⁴, HUANG Jiaqi¹, ZHANG Qiang²

1. Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology, Beijing 100081, P. R. China;
2. Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, P. R. China;
3. Beijing Key Laboratory of Lignocellulosic Chemistry, Beijing Forestry University, Beijing 100083, P. R. China;
4. School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006, P. R. China

Received:2020-04-11 Revised:2020-05-01 Online:2020-06-01 Published:2020-05-30
Contact: ZHANG Qiang E-mail:zhang-qiang@mails.tsinghua.edu.cn
Supported by:
Supported by the National Natural Science Foundation of China(Nos.21808124, 21825501, U1801257), the National Key Research and Development Program of China(Nos.2016YFA0202500, 2016YFA0200102) and the China Postdoctoral Science Foundation(No.2019T120098).

摘要/Abstract

摘要： Sulfide-based solid-state electrolytes with ultrahigh lithium ion conductivities have been considered as the most promising electrolyte system to enable practical all-solid-state batteries. However, the practical applications of the sulfide-based all-solid-state batteries are hindered by severe interfacial issues as well as large-scale material preparation and battery fabrication problems. Liquid-involved interfacial treatments and preparation processes compatible with current battery manufacturing capable of improving electrode/electrolyte interface contacts and realizing the mass production of sulfide electrolytes and the scalable fabrication of sulfide-based battery component have attracted considerable attention. In this perspective, the current advances in liquid-involved treatments and processes in sulfide-based all-solid-state batteries are summarized. Then relative chemical mechanisms and existing challenges are included. Finally, future guidance is also proposed for sulfide-based batteries. Focusing on the sulfide-based all-solid-state batteries, we aim at providing a fresh insight on understandings towards liquid-involved processes and promoting the development of all-solid-state batteries with higher energy density and better safety.

关键词: Sulfide electrolyte, All-solid-state battery, Composite electrode, Liquid-involved materials processing, Energy material

Abstract: Sulfide-based solid-state electrolytes with ultrahigh lithium ion conductivities have been considered as the most promising electrolyte system to enable practical all-solid-state batteries. However, the practical applications of the sulfide-based all-solid-state batteries are hindered by severe interfacial issues as well as large-scale material preparation and battery fabrication problems. Liquid-involved interfacial treatments and preparation processes compatible with current battery manufacturing capable of improving electrode/electrolyte interface contacts and realizing the mass production of sulfide electrolytes and the scalable fabrication of sulfide-based battery component have attracted considerable attention. In this perspective, the current advances in liquid-involved treatments and processes in sulfide-based all-solid-state batteries are summarized. Then relative chemical mechanisms and existing challenges are included. Finally, future guidance is also proposed for sulfide-based batteries. Focusing on the sulfide-based all-solid-state batteries, we aim at providing a fresh insight on understandings towards liquid-involved processes and promoting the development of all-solid-state batteries with higher energy density and better safety.

Key words: Sulfide electrolyte, All-solid-state battery, Composite electrode, Liquid-involved materials processing, Energy material

YUAN Hong, LIU Jia, LU Yang, ZHAO Chenzi, CHENG Xinbing, NAN Haoxiong, LIU Quanbing, HUANG Jiaqi, ZHANG Qiang. Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review[J]. 高等学校化学研究, 2020, 36(3): 377-385.

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Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review

Toward Practical All-solid-state Batteries with Sulfide Electrolyte: A Review

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