Recent Advances in 0D Ni/Co-based Hollow Electrocatalysts for Electrochemical Water Splitting

doi:10.1007/s40242-024-3278-3

高等学校化学研究 ›› 2024, Vol. 40 ›› Issue (3): 437-450.doi: 10.1007/s40242-024-3278-3

Recent Advances in 0D Ni/Co-based Hollow Electrocatalysts for Electrochemical Water Splitting

GE Wenjing, CHEN Xiaocui, MA Ruizhao, ZHENG Siyuan, SHANG Ningzhao, ZHAO Xiaoxian

Department of Chemistry, College of Science, Hebei Agricultural University, Baoding 071001, P. R. China

收稿日期:2023-12-19 出版日期:2024-06-01 发布日期:2024-06-01
通讯作者: ZHAO Xiaoxian,E-mail:lxzhxx@hebau.edu.cn E-mail:lxzhxx@hebau.edu.cn
基金资助:
This work was supported by the Talent Introduction Program of Hebei Agricultural University, China (No. YJ201810), the Youth Top-notch Talent Foundation of Hebei Provincial Universities, China (No. BJK2022023), the National Natural Science Foundation of China (NSFC) (No. 22105059), the Natural Science Foundation of Hebei Province, China (No. B2023204006), and the Talent Training Project of Hebei Province, China (No. A201901046).

Recent Advances in 0D Ni/Co-based Hollow Electrocatalysts for Electrochemical Water Splitting

GE Wenjing, CHEN Xiaocui, MA Ruizhao, ZHENG Siyuan, SHANG Ningzhao, ZHAO Xiaoxian

Department of Chemistry, College of Science, Hebei Agricultural University, Baoding 071001, P. R. China

Received:2023-12-19 Online:2024-06-01 Published:2024-06-01
Contact: ZHAO Xiaoxian,E-mail:lxzhxx@hebau.edu.cn E-mail:lxzhxx@hebau.edu.cn
Supported by:
This work was supported by the Talent Introduction Program of Hebei Agricultural University, China (No. YJ201810), the Youth Top-notch Talent Foundation of Hebei Provincial Universities, China (No. BJK2022023), the National Natural Science Foundation of China (NSFC) (No. 22105059), the Natural Science Foundation of Hebei Province, China (No. B2023204006), and the Talent Training Project of Hebei Province, China (No. A201901046).

摘要/Abstract

摘要： Electrochemical water splitting using renewable energy sources has been recognized as a sustainable way to produce hydrogen energy due to the characteristics of low-carbon and no pollution. However, the slow hydrogen/oxygen evolution reactions (HER/OER) seriously hinder the practical application of large-scale water splitting. In this paper, the 0D Ni/Co-based hollow material is discussed in detail because of adjustable morphology, low mass density and abundant active sites, which provides an effective solution for improving the HER/OER reaction kinetics. The synthesis methods of hollow materials, such as hard template, soft template and self-template are introduced. Afterward, catalysts with different structural designs of hollow structures are reviewed, including hollow single-shelled structure, hollow core-shelled structure, hollow double-shelled structure and hollow multi-shelled structure (HoMS) catalysts. Wherein, the research progress of the 0D Ni/Co-based HoMS electrocatalysts in recent years and their prominent performances in water splitting are highlighted. Finally, the challenges and development prospects of designing Ni/Co-based HoMS catalysts in water splitting in the future are discussed.

关键词: Electrochemical water splitting, Morphological regulation, Hollow structure, Hollow multi-shelled structure (HoMS)

Abstract: Electrochemical water splitting using renewable energy sources has been recognized as a sustainable way to produce hydrogen energy due to the characteristics of low-carbon and no pollution. However, the slow hydrogen/oxygen evolution reactions (HER/OER) seriously hinder the practical application of large-scale water splitting. In this paper, the 0D Ni/Co-based hollow material is discussed in detail because of adjustable morphology, low mass density and abundant active sites, which provides an effective solution for improving the HER/OER reaction kinetics. The synthesis methods of hollow materials, such as hard template, soft template and self-template are introduced. Afterward, catalysts with different structural designs of hollow structures are reviewed, including hollow single-shelled structure, hollow core-shelled structure, hollow double-shelled structure and hollow multi-shelled structure (HoMS) catalysts. Wherein, the research progress of the 0D Ni/Co-based HoMS electrocatalysts in recent years and their prominent performances in water splitting are highlighted. Finally, the challenges and development prospects of designing Ni/Co-based HoMS catalysts in water splitting in the future are discussed.

Key words: Electrochemical water splitting, Morphological regulation, Hollow structure, Hollow multi-shelled structure (HoMS)

GE Wenjing, CHEN Xiaocui, MA Ruizhao, ZHENG Siyuan, SHANG Ningzhao, ZHAO Xiaoxian. Recent Advances in 0D Ni/Co-based Hollow Electrocatalysts for Electrochemical Water Splitting[J]. 高等学校化学研究, 2024, 40(3): 437-450.

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Recent Advances in 0D Ni/Co-based Hollow Electrocatalysts for Electrochemical Water Splitting

Recent Advances in 0D Ni/Co-based Hollow Electrocatalysts for Electrochemical Water Splitting

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