Recent Advances in Atomic-scale Storage Mechanism Studies of Two-dimensional Nanomaterials for Rechargeable Batteries Beyond Li-ion

doi:10.1007/s40242-020-0187-y

高等学校化学研究 ›› 2020, Vol. 36 ›› Issue (4): 560-583.doi: 10.1007/s40242-020-0187-y

Recent Advances in Atomic-scale Storage Mechanism Studies of Two-dimensional Nanomaterials for Rechargeable Batteries Beyond Li-ion

PAN Lu^1,2, DONG Jinyang³, YI Ding¹, YANG Yijun¹, WANG Xi^1,2

1. Department of Physics, School of Science, Beijing Jiaotong University, Beijing 100044, P. R. China;
2. Chemistry and Chemical Engineering Guangdong Laboratory, Shantou 515031, P. R. China;
3. Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing 100081, P. R. China

收稿日期:2020-06-15 修回日期:2020-06-30 出版日期:2020-08-01 发布日期:2020-07-30
通讯作者: WANG Xi E-mail:xiwang@bjtu.edu.cn.
基金资助:
Supported by the Fundamental Research Funds for the Central Universities of China(No.2018JBZ107), the Key Program for International S&T Cooperation Projects of China(No.2018YFE0124600), the National Natural Science Foundation of China (Nos. 91961125, 21903001), and the Funds of the Chemistry and Chemical Engineering Guangdong Laboratory, China(No.1932004).

Recent Advances in Atomic-scale Storage Mechanism Studies of Two-dimensional Nanomaterials for Rechargeable Batteries Beyond Li-ion

PAN Lu^1,2, DONG Jinyang³, YI Ding¹, YANG Yijun¹, WANG Xi^1,2

1. Department of Physics, School of Science, Beijing Jiaotong University, Beijing 100044, P. R. China;
2. Chemistry and Chemical Engineering Guangdong Laboratory, Shantou 515031, P. R. China;
3. Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science and Engineering, Beijing Institute of Technology, Beijing 100081, P. R. China

Received:2020-06-15 Revised:2020-06-30 Online:2020-08-01 Published:2020-07-30
Contact: WANG Xi E-mail:xiwang@bjtu.edu.cn.
Supported by:
Supported by the Fundamental Research Funds for the Central Universities of China(No.2018JBZ107), the Key Program for International S&T Cooperation Projects of China(No.2018YFE0124600), the National Natural Science Foundation of China (Nos. 91961125, 21903001), and the Funds of the Chemistry and Chemical Engineering Guangdong Laboratory, China(No.1932004).

摘要/Abstract

摘要： Developing new types of rechargeable batteries with high energy densities and low cost have received increasing attentions, aiming to reduce the dependence on high-priced lithium. Beyond Li-ion batteries, the potential alternatives including Na-ion batteries, Li-S batteries and Li-air batteries have been investigated recently, which are required to be viable for commercial applications. From this point of view, to understand the electrochemical reaction mechanisms and kinetics of these batteries has become the key challenge to make breakthroughs in the field of new energy storage. In this review, we present a critical overview of the two dimensional nanomaterials-based batteries (except Li-ion-based batteries) that could meet such demonds. To develop new energy storage devices with more promising performances, the microstructure evolution and atomic scale storage mechanism of these batteries are comprehensively summarized. In addition, the major challenges and opportunities of advanced characterization techniques are finally discussed. We do hope that this review will give the readers a clear and profound understanding of the electrochemical reaction mechanisms and kinetics of the as-discussed batteries, thus effectively contributing to the smart design of future-generation energy storage devices.

关键词: Two dimensional (2D) nanomaterial, Batteries beyond Li ion, In situ technique, Atomic-level, Storage mechanism and kinetics

Abstract: Developing new types of rechargeable batteries with high energy densities and low cost have received increasing attentions, aiming to reduce the dependence on high-priced lithium. Beyond Li-ion batteries, the potential alternatives including Na-ion batteries, Li-S batteries and Li-air batteries have been investigated recently, which are required to be viable for commercial applications. From this point of view, to understand the electrochemical reaction mechanisms and kinetics of these batteries has become the key challenge to make breakthroughs in the field of new energy storage. In this review, we present a critical overview of the two dimensional nanomaterials-based batteries (except Li-ion-based batteries) that could meet such demonds. To develop new energy storage devices with more promising performances, the microstructure evolution and atomic scale storage mechanism of these batteries are comprehensively summarized. In addition, the major challenges and opportunities of advanced characterization techniques are finally discussed. We do hope that this review will give the readers a clear and profound understanding of the electrochemical reaction mechanisms and kinetics of the as-discussed batteries, thus effectively contributing to the smart design of future-generation energy storage devices.

Key words: Two dimensional (2D) nanomaterial, Batteries beyond Li ion, In situ technique, Atomic-level, Storage mechanism and kinetics

PAN Lu, DONG Jinyang, YI Ding, YANG Yijun, WANG Xi. Recent Advances in Atomic-scale Storage Mechanism Studies of Two-dimensional Nanomaterials for Rechargeable Batteries Beyond Li-ion[J]. 高等学校化学研究, 2020, 36(4): 560-583.

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Recent Advances in Atomic-scale Storage Mechanism Studies of Two-dimensional Nanomaterials for Rechargeable Batteries Beyond Li-ion

Recent Advances in Atomic-scale Storage Mechanism Studies of Two-dimensional Nanomaterials for Rechargeable Batteries Beyond Li-ion

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