Fabrication and Application of Graphdiyne-based Heterogeneous Compositions: from the View of Interaction

doi:10.1007/s40242-021-1362-5

高等学校化学研究 ›› 2021, Vol. 37 ›› Issue (6): 1158-1175.doi: 10.1007/s40242-021-1362-5

Fabrication and Application of Graphdiyne-based Heterogeneous Compositions: from the View of Interaction

QI Qi^1,2, XU Lekai³, DU Jiang^1,2, YANG Nailiang^3,4, WANG Dan^3,4

1. School of Materials Science and Engineering, Henan Province Industrial Technology Research Institute of Resources and Materials, Zhengzhou University, Zhengzhou 450001, P. R. China;
2. Green Catalysis Center, College of Chemistry, Zhengzhou University, Zhengzhou 450000, P. R. China;
3. State Key Laboratory of Biochemical Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, P. R. China;
4. University of Chinese Academy of Sciences, Beijing 100049, P. R. China

收稿日期:2021-09-10 修回日期:2021-10-09 出版日期:2021-11-23 发布日期:2021-10-25
通讯作者: DU Jiang, YANG Nailiang, WANG Dan E-mail:dj@zzu.edu.cn;nlyang@ipe.ac.cn;danwang@ipe.ac.cn
基金资助:
This work was supported by the National Key R&D Program of China (No.2018YFA0703504), the National Natural Science Foundation of China(Nos. 21971244, 51932001, 52174387) and the Project of the Education Department of Henan Province, China(No.20A430024).

Fabrication and Application of Graphdiyne-based Heterogeneous Compositions: from the View of Interaction

QI Qi^1,2, XU Lekai³, DU Jiang^1,2, YANG Nailiang^3,4, WANG Dan^3,4

1. School of Materials Science and Engineering, Henan Province Industrial Technology Research Institute of Resources and Materials, Zhengzhou University, Zhengzhou 450001, P. R. China;
2. Green Catalysis Center, College of Chemistry, Zhengzhou University, Zhengzhou 450000, P. R. China;
3. State Key Laboratory of Biochemical Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, P. R. China;
4. University of Chinese Academy of Sciences, Beijing 100049, P. R. China

Received:2021-09-10 Revised:2021-10-09 Online:2021-11-23 Published:2021-10-25
Contact: DU Jiang, YANG Nailiang, WANG Dan E-mail:dj@zzu.edu.cn;nlyang@ipe.ac.cn;danwang@ipe.ac.cn
Supported by:
This work was supported by the National Key R&D Program of China (No.2018YFA0703504), the National Natural Science Foundation of China(Nos. 21971244, 51932001, 52174387) and the Project of the Education Department of Henan Province, China(No.20A430024).

摘要/Abstract

摘要： Graphdiyne(GDY) has the unique feature in the topological ordered arranged sp- and sp²-hybridized carbon atoms, thus deriving a series of 2D allotropes. Due to inhomogeneous π-bonding and carbon orbital overlap between different hybrid carbon atoms, GDY possesses a natural band gap with a Dirac cones structure. And GDY exhibits semiconductor property with a conductivity of 2.516×10^-4 S/m at room temperature. The topological distribution of alkyne and benzene bonds of GDY makes its surface charge distribution extremely uneven, which produces high intrinsic activity for further modification. Its unique molecular structure endows the specific interaction with various species, such as ions, atoms, molecules and nanoparticles, showing excellent charge transport capability and unique advantages in mass transfer and energy conversion. From the view of the interaction principle between GDY and different compositions, we summarized the application of GDY-based materials in the fields of catalysis, energy conversion and storage, biological detection and so on.

关键词: Graphdiyne, Two-dimensional material, Carbon material, Interaction, Hetero-composition

Abstract: Graphdiyne(GDY) has the unique feature in the topological ordered arranged sp- and sp²-hybridized carbon atoms, thus deriving a series of 2D allotropes. Due to inhomogeneous π-bonding and carbon orbital overlap between different hybrid carbon atoms, GDY possesses a natural band gap with a Dirac cones structure. And GDY exhibits semiconductor property with a conductivity of 2.516×10^-4 S/m at room temperature. The topological distribution of alkyne and benzene bonds of GDY makes its surface charge distribution extremely uneven, which produces high intrinsic activity for further modification. Its unique molecular structure endows the specific interaction with various species, such as ions, atoms, molecules and nanoparticles, showing excellent charge transport capability and unique advantages in mass transfer and energy conversion. From the view of the interaction principle between GDY and different compositions, we summarized the application of GDY-based materials in the fields of catalysis, energy conversion and storage, biological detection and so on.

Key words: Graphdiyne, Two-dimensional material, Carbon material, Interaction, Hetero-composition

QI Qi, XU Lekai, DU Jiang, YANG Nailiang, WANG Dan. Fabrication and Application of Graphdiyne-based Heterogeneous Compositions: from the View of Interaction[J]. 高等学校化学研究, 2021, 37(6): 1158-1175.

QI Qi, XU Lekai, DU Jiang, YANG Nailiang, WANG Dan. Fabrication and Application of Graphdiyne-based Heterogeneous Compositions: from the View of Interaction[J]. Chemical Research in Chinese Universities, 2021, 37(6): 1158-1175.

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Fabrication and Application of Graphdiyne-based Heterogeneous Compositions: from the View of Interaction

Fabrication and Application of Graphdiyne-based Heterogeneous Compositions: from the View of Interaction

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