Challenges and Development of Composite Solid Electrolytes for All-solid-state Lithium Batteries

doi:10.1007/s40242-021-0007-z

高等学校化学研究 ›› 2021, Vol. 37 ›› Issue (2): 210-231.doi: 10.1007/s40242-021-0007-z

Challenges and Development of Composite Solid Electrolytes for All-solid-state Lithium Batteries

LIU Li, ZHANG Dechao, XU Xijun, LIU Zhengbo, LIU Jun

Guangdong Provincial Key Laboratory of Advanced Energy Storage Ma-te-rials, School of Materials Science and Engineering, South China University of Technology, Guangzhou 510641, P. R. China

收稿日期:2021-01-04 出版日期:2021-04-01 发布日期:2021-02-25
通讯作者: LIU Jun E-mail:msjliu@scut.edu.cn
基金资助:
This work was supported by the National Natural Science Foundation of China (No.51771076), the Guangdong “Pearl River Talents Plan” of China(No. 2017GC010218), the Guangdong Basic and Applied Basic Research Foundation, China(No.2020B1515120049) and the R&D Program in Key Areas of Guangdong Province of China(No.2020B0101030005).

Challenges and Development of Composite Solid Electrolytes for All-solid-state Lithium Batteries

LIU Li, ZHANG Dechao, XU Xijun, LIU Zhengbo, LIU Jun

Guangdong Provincial Key Laboratory of Advanced Energy Storage Ma-te-rials, School of Materials Science and Engineering, South China University of Technology, Guangzhou 510641, P. R. China

Received:2021-01-04 Online:2021-04-01 Published:2021-02-25
Contact: LIU Jun E-mail:msjliu@scut.edu.cn
Supported by:
This work was supported by the National Natural Science Foundation of China (No.51771076), the Guangdong “Pearl River Talents Plan” of China(No. 2017GC010218), the Guangdong Basic and Applied Basic Research Foundation, China(No.2020B1515120049) and the R&D Program in Key Areas of Guangdong Province of China(No.2020B0101030005).

摘要/Abstract

摘要： All-solid-state lithium batteries are considered to be a new battery system with great development potential and application prospects due to the advantages of high energy density and high security. As a key component of all-solid-state lithium batteries, the development of solid-state electrolytes has received extensive attention in recent years, but most solid electrolytes still exhibit problems, such as low ion conductivity and poor interface compatibility. The design of composite solid-state electrolyte materials with both excellent electrochemical and mechanical properties is an effective way to develop all-solid-state lithium batteries. This review introduces different types of pure component solid electrolytes and analyzes their respective advantages and characteristics firstly. Furthermore, the research progress of composite electrolytes in preparation method, ionic conduction, suppression of lithium dendrites, and the improvement of electrochemical performances are reviewed from the perspective of composite electrolyte structure design, which is to meet different performance requirements. And the future development direction and trend of composite electrolytes are prospected.

关键词: All-solid-state lithium battery, Solid electrolyte, Composite solid electrolyte

Abstract: All-solid-state lithium batteries are considered to be a new battery system with great development potential and application prospects due to the advantages of high energy density and high security. As a key component of all-solid-state lithium batteries, the development of solid-state electrolytes has received extensive attention in recent years, but most solid electrolytes still exhibit problems, such as low ion conductivity and poor interface compatibility. The design of composite solid-state electrolyte materials with both excellent electrochemical and mechanical properties is an effective way to develop all-solid-state lithium batteries. This review introduces different types of pure component solid electrolytes and analyzes their respective advantages and characteristics firstly. Furthermore, the research progress of composite electrolytes in preparation method, ionic conduction, suppression of lithium dendrites, and the improvement of electrochemical performances are reviewed from the perspective of composite electrolyte structure design, which is to meet different performance requirements. And the future development direction and trend of composite electrolytes are prospected.

Key words: All-solid-state lithium battery, Solid electrolyte, Composite solid electrolyte

LIU Li, ZHANG Dechao, XU Xijun, LIU Zhengbo, LIU Jun. Challenges and Development of Composite Solid Electrolytes for All-solid-state Lithium Batteries[J]. 高等学校化学研究, 2021, 37(2): 210-231.

LIU Li, ZHANG Dechao, XU Xijun, LIU Zhengbo, LIU Jun. Challenges and Development of Composite Solid Electrolytes for All-solid-state Lithium Batteries[J]. Chemical Research in Chinese Universities, 2021, 37(2): 210-231.

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Challenges and Development of Composite Solid Electrolytes for All-solid-state Lithium Batteries

Challenges and Development of Composite Solid Electrolytes for All-solid-state Lithium Batteries

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